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The First Catalytic Synthesis of an Acrylate from CO2 and an Alkene—A Rational Approach
Abstract
For more than three decades the catalytic synthesis of acrylates from the cheap and abundantly available C 1 building block carbon dioxide and alkenes has been an unsolved problem in catalysis research, both in academia and industry. Herein, we describe a homogeneous catalyst based on nickel that permits the catalytic synthesis of the industrially highly relevant acrylate sodium acrylate from CO 2, ethylene, and a base, as demonstrated, at this stage, by a turnover number of greater than 10 with respect to the metal.
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Citations
Cited by
Klankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
Sustainable conversion of carbon dioxide: the advent of organocatalysis
Fiorani, G., Guo, W., & Kleij, A. W. (2015) · Green Chemistry · doi:10.1039/c4gc01959h · Cited by 658
Ostapowicz, T. G., Schmitz, M., Krystof, M., Klankermayer, J., & Leitner, W. (2013) · Angewandte Chemie · doi:10.1002/ange.201304529 · Cited by 63
Catalytic conversion of carbon dioxide to carboxylic acid derivatives
Liu, A., Yu, B., & He, L. (2015) · Greenhouse Gases Science and Technology · doi:10.1002/ghg.1461 · Cited by 57
Metadata
- Authors
- Lejkowski, M. L., Lindner, R., Kageyama, T., Bódizs, G. É., Plessow, P. N., Müller, I. B., Schäfer, A., Rominger, F., Hofmann, P., Futter, C., Schunk, S. A., & Limbach, M.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2012-09-20
- Volume
- 18
- Issue
- 44
- Pages
- 14017-14025
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2166617552
- Cited by
- 205
- References
- 0
- FWCI
- 10.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: The First Catalytic Synthesis of an Acrylate from CO2 and an Alkene—A Rational Approach. https://app.cochat.ai/papers/10.1002/chem.201201757
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- Lejkowski, M. L., Lindner, R., Kageyama, T., Bódizs, G. É., Plessow, P. N., Müller, I. B., Schäfer, A., Rominger, F., Hofmann, P., Futter, C., Schunk, S. A., & Limbach, M. (2012). The First Catalytic Synthesis of an Acrylate from CO2 and an Alkene—A Rational Approach. Chemistry – A European Journal. https://doi.org/10.1002/chem.201201757
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
