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Highly Efficient Hydrogen Storage System Based on Ammonium Bicarbonate/Formate Redox Equilibrium over Palladium Nanocatalysts
Abstract
A highly efficient, reversible hydrogen storage–evolution process has been developed based on the ammonium bicarbonate/formate redox equilibrium over the same carbon‐supported palladium nanocatalyst. This heterogeneously catalyzed hydrogen storage system is comparable to the counterpart homogeneous systems and has shown fast reaction kinetics of both the hydrogenation of ammonium bicarbonate and the dehydrogenation of ammonium formate under mild operating conditions. By adjusting temperature and pressure, the extent of hydrogen storage and evolution can be well controlled in the same catalytic system. Moreover, the hydrogen storage system based on aqueous‐phase ammonium formate is advantageous owing to its high volumetric energy density.
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Electrocatalyst approaches and challenges for automotive fuel cells
Debe, M. K. (2012) · Nature · doi:10.1038/nature11115 · Cited by 5,885
Photocatalytic Water Splitting: Recent Progress and Future Challenges
Maeda, K., & Domen, K. (2010) · The Journal of Physical Chemistry Letters · doi:10.1021/jz1007966 · Cited by 2,739
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Formic Acid-Based Liquid Organic Hydrogen Carrier System with Heterogeneous Catalysts
Zhong, H., Iguchi, M., Chatterjee, M., Himeda, Y., Xu, Q., & Kawanami, H. (2018) · Advanced Sustainable Systems · doi:10.1002/adsu.201700161 · Cited by 209
Estevez, R., López-Tenllado, F. J., Aguado-Deblas, L., Bautista, F. M., Romero, A. A., & Luna, D. (2023) · Energies · doi:10.3390/en16145451 · Cited by 55
Enhancing H2 evolution by optimizing H adatom combination and desorption over Pd nanocatalyst
Wang, J., Tan, H., Jiang, D., & Zhou, K. (2017) · Nano Energy · doi:10.1016/j.nanoen.2017.02.001 · Cited by 54
Metadata
- Authors
- Su, J., Yang, L., Lu, M., & Lin, H.
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2015-02-06
- Volume
- 8
- Issue
- 5
- Pages
- 813-816
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2145466975
- Cited by
- 180
- References
- 2
- FWCI
- 3.60
- Type
- journal article
- Language
- en
- Open access
- closed
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