Carbon Foam Decorated with Silver Nanoparticles for Electrochemical CO2 Conversion
Open accessAbstract
Electrochemistry is a promising method to recycle CO 2 into useful carbon feedstock and for storing intermittent renewable energy. To date, Au and Ag nanoparticles are the most active catalysts for electrochemical conversion of CO 2 to CO. However, agglomeration reduces the activity and the high cost slows widespread commercialization. Suitable support materials are thus needed to improve catalyst utilization. We explore carbon foam (CF) as a catalyst support. Compared with carbon black or graphene nanoplatelets, CF has higher surface area, larger pores, and more defects, resulting in improved uniformity of Ag nanoparticle distribution as well as higher activity and efficiency for CO 2 conversion to CO.
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There is a distinction between bulk electrolyte pH and local cathode pH, as reduction reactions drive up the local pH at the electrode surface.
“There is a distinction between bulk electrolyte pH and local cathode pH, as reduction reactions drive up the local pH at the electrode surface.[199]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [199]
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- Authors
- Ma, S., Liu, J., Sasaki, K., Lyth, S. M., & Kenis, P. J. A.
- Affiliations
- Kyushu University (JP)
- Corresponding author
- Lyth, Stephen M.
- Kenis, Paul J. A.
- Venue
- Energy Technology
- Publisher
- Wiley
- Published
- 2017-01-25
- Volume
- 5
- Issue
- 6
- Pages
- 861-863
- ISSN
- 2194-4288 (ISSN-L)
- 2194-4296
- OpenAlex
- W2557778878
- Cited by
- 45
- References
- 21
- Citations by year
- 2026: 2 · 2025: 1 · 2024: 3 · 2023: 2 · 2022: 4 · 2021: 9 · 2020: 8 · 2019: 9 · 2018: 4 · 2017: 3
- FWCI
- 1.45
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Energy Technology (publishedVersion)
- Strathprints: The University of Strathclyde institutional repository (University of Strathclyde) (acceptedVersion)
- Funders
- International Institute for Carbon-Neutral Energy Research, Kyushu University (WPI–I2CNER)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- carbon foam, silver nanoparticles, electrochemical CO2 reduction, CO2 to CO conversion, catalyst supports, nanoparticle agglomeration, carbon black, graphene nanoplatelets, surface area
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