The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Sustainion Imidazolium‐Functionalized Polymers for Carbon Dioxide Electrolysis
Open accessAbstract
CO 2 electrolysis is a key step in CO 2 conversion into fuels and chemicals as a way of mitigating climate change. We report the synthesis and testing of a series of new anion‐conductive membranes (tradenamed Sustainion™) for use in CO 2 electrolysis. These membranes incorporate the functional character of imidazolium‐based ionic liquids as co‐catalysts in CO 2 reduction into a solid membrane with a styrene backbone. We find that the addition of an imidazolium group onto the styrene side‐chains increases the selectivity of the reaction from approximately 25 % to approximately 95 %. The current at 3 V is increased by a factor of 14. So far we have been able to tune these parameters to achieve stable cells that provide current densities higher than 100 mA cm−2 at 3 V cell potential with a CO product selectivity over 98 %. Stable performance was observed for 6 months of continuous operation (>150 000 000 turnovers). These results demonstrate that imidazolium polymers are ideal membranes for CO 2 electrolysis.
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Cites
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
Rosen, B. A., Salehi-Khojin, A., Thorson, M. R., Zhu, W., Whipple, D. T., Kenis, P. J. A., & Masel, R. I. (2011) · Science · doi:10.1126/science.1209786 · Cited by 1,558
Self-citationVerma, S., Lu, X., Ma, S., Masel, R. I., & Kenis, P. J. A. (2016) · Physical Chemistry Chemical Physics · doi:10.1039/c5cp05665a · Cited by 497
Self-citationLim, R. J., Xie, M., Sk, M. A., Lee, J.-M., Fisher, A., Wang, X., & Lim, K. H. (2014) · Catalysis Today · doi:10.1016/j.cattod.2013.11.037 · Cited by 460
Effect of solid polymer electrolyte on electrochemical reduction of CO2
Aeshala, L. M., Rahman, S. U., & Verma, A. (2012) · Separation and Purification Technology · doi:10.1016/j.seppur.2011.12.030 · Cited by 89
Cited by
CO 2 electrolysis to multicarbon products in strong acid
Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., et al. (2021) · Science · doi:10.1126/science.abg6582 · Cited by 1,359
Kibria, M. G., Edwards, J. P., Gabardo, C. M., Dinh, C., Seifitokaldani, A., Sinton, D., & Sargent, E. H. (2019) · Advanced Materials · doi:10.1002/adma.201807166 · Cited by 1,331
Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
Zheng, T., Jiang, K., Ta, N., Hu, Y., Zeng, J., Liu, J., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.10.015 · Cited by 887
Garg, S., Li, M., Weber, A. Z., Ge, L., Li, L., Rudolph, V., Wang, G., & Rufford, T. E. (2020) · Journal of Materials Chemistry A · doi:10.1039/c9ta13298h · Cited by 478
Endrődi, B., Kecsenovity, E., Samu, A., Halmágyi, T., Rojas-Carbonell, S., Wang, L., Yan, Y., & Janáky, C. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02589e · Cited by 303
Metadata
- Authors
- Kutz, R. B., Chen, Q., Yang, H., Sajjad, S. D., Liu, Z., & Masel, I. R.
- Venue
- Energy Technology
- Publisher
- Wiley
- Published
- 2017-03-09
- Volume
- 5
- Issue
- 6
- Pages
- 929-936
- ISSN
- 2194-4288 (ISSN-L)
- 2194-4296
- OpenAlex
- W2561463699
- Cited by
- 427
- References
- 5
- FWCI
- 4.56
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Kutz, R. B., Chen, Q., Yang, H., Sajjad, S. D., Liu, Z., & Masel, I. R. (2017). Sustainion Imidazolium‐Functionalized Polymers for Carbon Dioxide Electrolysis. Energy Technology. https://doi.org/10.1002/ente.201600636
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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