Deformable, transparent, high‐performance, room‐temperature oxygen sensors based on ion‐conductive, environment‐tolerant, and green organohydrogels
Open accessAbstract
We present green organohydrogel‐based stretchable (up to 700% strain), transparent, and room‐temperature O 2 sensors with impressive performance, including drying and freezing tolerances, high sensitivity, broad detection range (100 ppm‐100%), long‐term stability, low theoretical detection limit (0.585 ppm), linearity, and the capability to real‐time monitor human respiration by directly attaching on human skin. A facile solvent replacement approach is employed to partially exchange water with natural and edible xylitol/sorbitol molecules, generating stable, green and tough organohydrogels. Compared with the pristine hydrogel counterpart, the organohydrogel‐based O 2 sensors feature higher stability, prolonged life time (140 days) and the ability to work over a wide range of temperatures (−38 to 65°C). The O 2 sensing mechanism is elucidated by investigating the redox reactions occurred at the electrode‐hydrogel interface. This work develops a facile strategy to fabricate stretchable, transparent, and high‐performance O 2 sensor using stable and green organohydrogels as novel transducing materials for practical wearable applications. image
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Recent studies have reported the use of hydrogels as the sensitive material for gas-sensing applications such as NO2, NH3, CO2, and O2.
“Recent studies have reported the use of hydrogels as the sensitive material for gas-sensing applications, such as NO2, NH3, CO2, and O2”
From Functionalized Hydrogel-Based Wearable Gas and Humidity Sensors. (2023) · cites this paper as [75]
Cites
Highly stretchable electroluminescent skin for optical signaling and tactile sensing
Larson, C., Peele, B., Li, S., Robinson, S., Totaro, M., Beccai, L., Mazzolai, B., & Shepherd, R. (2016) · Science · doi:10.1126/science.aac5082 · Cited by 1,393 · see citing works
Wu, J., Wu, Z., Xu, H., Wu, Q., Liu, C., Yang, B.-R., Gui, X., Xie, X., Tao, K., Shen, Y., et al. (2019) · Materials Horizons · doi:10.1039/c8mh01160e · Cited by 391 · see citing works
Self-citationWu, J., Wu, Z., Han, S., Yang, B.-R., Gui, X., Tao, K., Liu, C., Miao, J., & Norford, L. K. (2019) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.8b17437 · Cited by 225 · see citing works
Self-citationWu, Z., Shi, W., Ding, H., Zhong, B., Huang, W., Zhou, Y., Gui, X., Xie, X., & Wu, J. (2021) · Journal of Materials Chemistry C · doi:10.1039/d1tc02506f · Cited by 121 · see citing works
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Functionalized Hydrogel-Based Wearable Gas and Humidity Sensors.
Luo, Y., Li, J., Ding, Q., Wang, H., Liu, C., & Wu, J. (2023) · Nano-Micro Letters · doi:10.1007/s40820-023-01109-2 · Cited by 236 · see citing works
“Recent studies have reported the use of hydrogels as the sensitive material for gas-sensing applications, such as NO 2 , NH 3 , CO 2 , and O 2 [67–75].”
BackgroundSelf-citation
- Authors
- Lin, Y., Wu, Z., Li, C., Ding, Q., Tao, K., Zhai, K., Chen, M., Zilberman, M., Xie, X., & Wu, J.
- Affiliations
- Sun Yat-sen University (CN)
- Northwestern Polytechnical University (CN)
- University of Macau (MO)
- Tel Aviv University (IL)
- Corresponding author
- Wu, Jin
- ORCID
- Venue
- EcoMat
- Publisher
- Wiley
- Published
- 2022-05-11
- Volume
- 4
- Issue
- 6
- ISSN
- 2567-3173 (ISSN-L)
- OpenAlex
- W4280612689
- Cited by
- 30
- References
- 4
- Citations by year
- 2026: 3 · 2025: 5 · 2024: 10 · 2023: 7 · 2022: 5
- FWCI
- 1.85
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- EcoMat (publishedVersion, cc-by)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- Basic and Applied Basic Research Foundation of Guangdong Province (2020A1515010693, 2021A1515110269)
- National Natural Science Foundation of China (61801525)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Gas Sensing Nanomaterials and Sensors
- Physical Sciences › Engineering › Biomedical Engineering › Advanced Sensor and Energy Harvesting Materials
- Physical Sciences › Chemical Engineering › Bioengineering › Analytical Chemistry and Sensors
- Keywords
- oxygen sensors, organohydrogel, stretchable sensors, transparent sensors, room-temperature sensing, solvent replacement, wearable electronics, respiratory monitoring, redox reactions
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