Advances and Applications of Metal‐Organic Frameworks (MOFs) in Emerging Technologies: A Comprehensive Review

Li, Dongxiao; Yadav, Anurag; Zhou, Hong; Roy, Kaustav; Thanasekaran, Pounraj; Lee, Chengkuo

doi:10.1002/gch2.202300244

Cited by 437Metal-Organic Frameworks: Synthesis and ApplicationsCovalent Organic Framework ApplicationsMembrane Separation and Gas Transport

Advances and Applications of Metal‐Organic Frameworks (MOFs) in Emerging Technologies: A Comprehensive Review

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Li, Dongxiao, Yadav, Anurag, Zhou, Hong, Roy, Kaustav, Thanasekaran, Pounraj, Lee, Chengkuo·2024·Global Challenges

DOI 10.1002/gch2.202300244PMC PMC10862192

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Abstract

Metal‐organic frameworks (MOFs) that are the wonder material of the 21st century consist of metal ions/clusters coordinated to organic ligands to form one‐ or more‐dimensional porous structures with unprecedented chemical and structural tunability, exceptional thermal stability, ultrahigh porosity, and a large surface area, making them an ideal candidate for numerous potential applications. In this work, the recent progress in the design and synthetic approaches of MOFs and explore their potential applications in the fields of gas storage and separation, catalysis, magnetism, drug delivery, chemical/biosensing, supercapacitors, rechargeable batteries and self‐powered wearable sensors based on piezoelectric and triboelectric nanogenerators are summarized. Lastly, this work identifies present challenges and outlines future opportunities in this field, which can provide valuable references.

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Regeneration efficiency varies widely among MOF frameworks, and large-scale production still requires substantial solvent and energy input, raising sustainability concerns.
“In addition, regeneration efficiency varies widely among frameworks, and large-scale production still requires substantial solvent and energy input, raising sustainability concerns.225–229”
From Emerging nanotechnology approaches for sustainable water treatment and heavy metals removal: a comprehensive review (2025) · cites this paper as [228]
The MOFs Preparation and Fabrication sections (pages unavailable) identify hazardous solvents in solvothermal synthesis and high energy consumption in mechanochemical synthesis, supporting concerns about production inputs. They do not establish that large-scale production generally requires substantial amounts of both, and the copy does not report that regeneration efficiency varies widely among frameworks (searched: regeneration and scale-up energy and solvent consumption). (LLM, conf=0.83)
Experimental — accuracy not yet measured
Fine MOF powders, though effective in batch adsorption, are unsuitable for continuous-flow systems due to high pressure drops and potential material loss.
“Fine MOF powders, though effective in batch adsorption, are unsuitable for continuous-flow systems due to high pressure drops and potential material loss.”
From Emerging nanotechnology approaches for sustainable water treatment and heavy metals removal: a comprehensive review (2025) · cites this paper as [228]
The Gas Storage and Separation in MOFs section describes MOFs as adsorbents and mentions packing efficiency as a practical issue, but does not address whether fine MOF powders work in batch adsorption or are unsuitable for continuous flow. Searches for pressure drop, material loss, fixed-bed operation, and batch adsorption found no passage supporting those specific claims. Page numbers were unavailable in our copy. (LLM, conf=0.73)
Experimental — accuracy not yet measured
Formulating MOFs into pellets, granules, or membranes often reduces accessible active sites.
“Thus, MOFs must be formulated into pellets, granules, or membranes, but these processes often reduce accessible active sites.”
From Emerging nanotechnology approaches for sustainable water treatment and heavy metals removal: a comprehensive review (2025) · cites this paper as [228]
The ‘MOFs Preparation and Fabrication’ sections discuss synthesis and membranes, while ‘Catalysis in MOFs’ discusses active sites; neither says that forming MOFs into pellets, granules, or membranes reduces access to those sites. Searches for pelletization, granules, shaping, and pore blocking found no passage addressing that claimed effect. Page numbers were not available in our copy. (LLM, conf=0.75)
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Authors: Li, D., Yadav, A., Zhou, H., Roy, K., Thanasekaran, P., & Lee, C.
Affiliations: National University of Singapore (SG)
Pondicherry University (IN)
Corresponding author: Thanasekaran, Pounraj
Lee, Chengkuo
ORCID: Li, Dongxiao
Zhou, Hong
Roy, Kaustav
Thanasekaran, Pounraj
Lee, Chengkuo
Venue: Global Challenges
Publisher: Wiley
Published: 2023-12-30
Volume: 8
Issue: 2
Pages: 2300244-2300244
ISSN: 2056-6646 (ISSN-L)
DOI: 10.1002/gch2.202300244
PMC: PMC10862192
OpenAlex: W4390451371
Cited by: 437
References: 288
Citations by year: 2026: 176 · 2025: 201 · 2024: 59 · 2023: 1
FWCI: 7.51
Type: journal article
Language: en
Open access: gold
doi.org
Licence: cc-by
creativecommons.org/licenses/by/4.0/ (vor)
Locations: Global Challenges (publishedVersion, cc-by)
PubMed Central (publishedVersion, cc-by)
PubMed (publishedVersion)
DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
Funders: Agency for Science, Technology and Research (A18A4b0055)
National Research Foundation Singapore (CRP28‐2022‐0038)
Advanced Research and Technology Innovation Centre, College of Design and Engineering, National University of Singapore (A‐0005947‐20‐00)
Ministry of Education (R‐263‐000‐F18‐112/A‐0009520‐01‐00)
Topics: Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
Physical Sciences › Materials Science › Materials Chemistry › Covalent Organic Framework Applications
Physical Sciences › Engineering › Mechanical Engineering › Membrane Separation and Gas Transport
Keywords: metal-organic frameworks, MOF synthesis, porous media, gas storage, gas separation, catalysis, magnetism, drug delivery, biosensing, chemical sensing, supercapacitors, rechargeable batteries, piezoelectric nanogenerators, triboelectric nanogenerator, wearable sensors, self-powered sensors

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