Shape memory behaviors of crosslinked copolymers containing stearyl acrylate
Abstract
Abstract Shape memory polymers were prepared by copolymerizing stearyl acrylate and methyl acrylate. The principle of this shape memory effect is based on reversible order‐disorder transition of crystalline aggregates of stearyl moieties. A specific feature of this type of shape memory copolymer is that the transition temperature at which the polymer abruptly becomes soft and deforms can be controlled by changing the monomer composition, which enables one to adjust the shape memory effect at a desired temperature. Mechanism and process of the shape memory behaviors were discussed.
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When activated after programming, either strain or stress recovery results from relaxation of temporarily fixed polymer chains, ascribed to entropy elasticity; the polymer restores its random coil conformation.
“When activated after programming, either strain or stress recovery results from the relaxation of temporarily “fixed” polymer chains, which can be ascribed to the phenomenon of entropy elasticity.Thus, the polymer restores its random coil conformation [69].”
From Review on the Functional Determinants and Durability of Shape Memory Polymers (2010) · cites this paper as [69]
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- Authors
- Kagami, Y., Gong, J. P., & Osada, Y.
- Affiliations
- Hokkaido University (JP)
- Corresponding author
- Osada, Yoshihito
- Venue
- Macromolecular Rapid Communications
- Publisher
- Wiley
- Published
- 1996-08
- Volume
- 17
- Issue
- 8
- Pages
- 539-543
- ISSN
- 1022-1336 (ISSN-L)
- 1521-3927
- OpenAlex
- W2016421336
- Cited by
- 99
- References
- 3
- Citations by year
- 2026: 1 · 2025: 1 · 2024: 2 · 2023: 5 · 2022: 5 · 2021: 3 · 2019: 12 · 2018: 3 · 2017: 8 · 2016: 7 · 2015: 3 · 2014: 3 · 2013: 5 · 2012: 3
- FWCI
- 1.03
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Macromolecular Rapid Communications (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
- Physical Sciences › Engineering › Mechanical Engineering › Advanced Materials and Mechanics
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Medicine › Hydrogels: synthesis, properties, applications
- Keywords
- shape memory polymers, stearyl acrylate, methyl acrylate, crosslinked copolymers, order-disorder transition, crystalline aggregates, monomer composition, shape memory mechanism
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