The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Defect Engineering Strategies for Nitrogen Reduction Reactions under Ambient Conditions
Abstract
The production of ammonia from N 2 molecules under ambient conditions [electro (photo) chemical reduction] is one of the most attractive topics in the energy‐related field due to its unique advantages and great potentials. Recently, various catalysts have been explored to show certain activities in nitrogen reduction reactions (NRRs) at room temperature and atmospheric pressure. To further improve the catalytic activity and increase the selectivity, the catalysts should be rationally designed to introduce extra active sites for the N 2 molecule adsorption and activation. This review summarizes recent progress of the defect engineering strategies to design highly efficient electrochemical or photocatalytic NRR nanocatalysts. The defect sites would serve as the active center for the NRR and further enhance its intrinsic performance. The defect engineering strategies are summarized in different categories, including vacancies (oxygen, nitrogen, and sulfur vacancies), doping (metal doping and nonmetal doping), amorphous phases (amorphous noble metal and amorphous transition metal), size effects, and structure effects. In addition, the different ammonia determination methods are summarized and compared in order to obtain more credible and veritable NRR performance results.
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Cites
Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts
Jaramillo, T. F., Jørgensen, K. P., Bonde, J., Nielsen, J. H., Horch, S., & Chorkendorff, I. (2007) · Science · doi:10.1126/science.1141483 · Cited by 6,100
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Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
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Cited by
Defect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Two-dimensional MXene-based and MXene-derived photocatalysts: Recent developments and perspectives
Zhong, Q., Li, Y., & Zhang, G. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2020.128099 · Cited by 466
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Wu, Y., Li, Y., Gao, J., & Zhang, Q. (2021) · SusMat · doi:10.1002/sus2.3 · Cited by 319
Metadata
- Authors
- Yan, D., Li, H., Chen, C., Zou, Y., & Wang, S.
- Venue
- Small Methods
- Publisher
- Wiley
- Published
- 2018-10-24
- Volume
- 3
- Issue
- 6
- ISSN
- 2366-9608 (ISSN-L)
- OpenAlex
- W2898376934
- Cited by
- 284
- References
- 4
- FWCI
- 7.30
- Type
- journal article
- Language
- en
- Open access
- closed
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