The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Rational design of donor-π-acceptor conjugated microporous polymers for photocatalytic hydrogen production
Abstract
Abstract Developing highly efficient catalysts for photocatalytic hydrogen generation from water splitting is one of the grand challenges in solar energy conversion. Herein, we report the design and synthesis of a library of donor-π-acceptor (D-π-A) conjugated microporous polymer (CMP) photocatalysts using pyrene, benzothiadiazole, and benzene (biphenyl) as donor, acceptor, and π crosslinker units, respectively. By adjusting the ratio of pyrene to benzothiadiazole units, a range of CMPs with various polymeric structures and components was synthesized and the influence of the molecular structures on the photocatalytic performance was comparatively investigated. Photocatalytic hydrogen evolution rate (HER) up to 106 μmol h–1 was achieved on PyBT-2 with a ratio of 9:2 of pyrene to benzothiadiazole under UV–vis light irradiation (λ > 300 nm). The structure-performance relationships revealed in this work offer a fundamental understanding in the rational design of CMPs for high performance organic photocatalysts.
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Citations
Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Graphene-based semiconductor photocatalysts
Xiang, Q., Yu, J., & Jaroniec, M. (2012) · Chem. Soc. Rev. · doi:10.1039/c1cs15172j · Cited by 2,730
Cited by
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Porous organic polymers: a promising platform for efficient photocatalysis
Zhang, T., Xing, G., Chen, W., & Chen, L. (2020) · Materials Chemistry Frontiers · doi:10.1039/c9qm00633h · Cited by 420
Bai, Y., Wilbraham, L., Slater, B. J., Zwijnenburg, M. A., Sprick, R. S., & Cooper, A. I. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03591 · Cited by 409
Lan, Z.-A., Ren, W., Chen, X., Zhang, Y., & Wang, X. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.01.010 · Cited by 265
Self-citationConjugated porous polymers: incredibly versatile materials with far-reaching applications
Taylor, D., Dalgarno, S. J., Xu, Z., & Vilela, F. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00315k · Cited by 259
Metadata
- Authors
- Xu, Y., Mao, N., Zhang, C., Wang, X., Zeng, J., Chen, Y., Wang, F., & Jiang, J.-X.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2018-07
- Volume
- 228
- Pages
- 1-9
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2793481353
- Cited by
- 290
- References
- 3
- FWCI
- 7.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, Y., Mao, N., Zhang, C., Wang, X., Zeng, J., Chen, Y., Wang, F., & Jiang, J.-X. (2018). Rational design of donor-π-acceptor conjugated microporous polymers for photocatalytic hydrogen production. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.01.073
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