The DOI matches its Crossref record; 45 of the 45 references it cites were found in a registry or an index.
Conjugated donor-acceptor polymer photocatalysts with electron-output “tentacles” for efficient hydrogen evolution
Abstract
Abstract The tunable structures and versatile properties for conjugated polymers (CPs) make them viable as a molecular platform for photocatalytic water splitting. Normally, structure design of polymer photocatalyst is focus on tuning its optical band structure or charge-separation ability, the importance of electron-output ability in photocatalytic process is always ignored. This study demonstrates a molecular engineering strategy by introducing an electron-output “tentacle” site, i.e. dibenzothiophene-S,S-dioxide (FSO) unit, into the polymer backbone to construct a series of donor-acceptor type conjugated polymer photocatalysts for efficient hydrogen evolution, which not only results in optimized light absorption ability and excellent exciton-separation, but also leads to the efficient electron-output ability. Detailed DFT calculations further theoretically confirm the vital role of FSO unit as an electron-output “tentacle” site.
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Cites
A metal-free polymeric photocatalyst for hydrogen production from water under visible light
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Self-citationHeterogeneous photocatalyst materials for water splitting
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Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
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Graphitic Carbon Nitride Polymers toward Sustainable Photoredox Catalysis
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Self-citationSulfone-containing covalent organic frameworks for photocatalytic hydrogen evolution from water
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Self-citationTunable Organic Photocatalysts for Visible-Light-Driven Hydrogen Evolution
Sprick, R. S., Jiang, J.-X., Bonillo, B., Ren, S., Ratvijitvech, T., Guiglion, P., Zwijnenburg, M. A., Adams, D. J., & Cooper, A. I. (2015) · Journal of the American Chemical Society · doi:10.1021/ja511552k · Cited by 896
Conjugated Polymers: Catalysts for Photocatalytic Hydrogen Evolution
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Cited by
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Metadata
- Authors
- Lan, Z.-A., Ren, W., Chen, X., Zhang, Y., & Wang, X.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2019-05
- Volume
- 245
- Pages
- 596-603
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2909687177
- Cited by
- 265
- References
- 45
- FWCI
- 6.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lan, Z.-A., Ren, W., Chen, X., Zhang, Y., & Wang, X. (2019). Conjugated donor-acceptor polymer photocatalysts with electron-output “tentacles” for efficient hydrogen evolution. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2019.01.010
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