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Cited by 285

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Engineering MoS2 nanomesh with holes and lattice defects for highly active hydrogen evolution reaction

Li, Yue, Yin, Kai, Wang, Longlu, Lu, Xiaolong, Zhang, Yaqi, Liu, Yutang, Yan, Dafeng, Song, Yuze, Luo, Shenglian·2018·Applied Catalysis B: Environmental
DOI 10.1016/j.apcatb.2018.05.080
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Abstract

Abstract Molybdenum disulfide (MoS2) presents a promising catalyst to replace state-of the-art platinum (Pt) for hydrogen evolution reaction (HER), but it still lacks an effective way due to the catalytically inert basal plane. Herein, we report a rational design of MoS2 nanomesh that possesses evenly distributed holes and defects to make full use of the 2H-MoS2 basal planes by combining ball-milling with ultrasonic methods. The exfoliation of muti-layer MoS2 to fewer layer or enven monolayer is proceed in pure water without using any chemicals or surfactants. The great advantage of the catalyst is the monolayer, holey and defective structure, which maximizing the synergistic activity for both electrocatalytic and photocatalytic HER performances. Impressively, the MoS2 nanomesh renders outstanding electrocatalytic HER activity with an overpotential of 160 mV at a current density of 10 mV cm−2, and a small Tafel slope of 46 mV decade−1. The photocatalytic H2 evolution rate is about 4.84 mmol h−1 when working with Eosin Y as an organic photosensitizer. Additionally, this catalyst shows excellent cycle stability in the electrochemical and photocatalytic reactions. This present work put a new insight into the large-scale production of chemically active 2H MoS2-based catalysts for HER.

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Metadata

Authors
Li, Y., Yin, K., Wang, L., Lu, X., Zhang, Y., Liu, Y., Yan, D., Song, Y., & Luo, S.
Venue
Applied Catalysis B: Environmental
Publisher
Elsevier BV
Published
2018-12
Volume
239
Pages
537-544
ISSN
0926-3373 (ISSN-L)
DOI
10.1016/j.apcatb.2018.05.080
OpenAlex
W2807291543
Cited by
285
References
3
FWCI
6.90
Type
journal article
Language
en
Open access
closed
Licence
  • www.elsevier.com/tdm/userlicense/1.0/ (tdm)
  • www.elsevier.com/legal/tdmrep-license (tdm)
Funders
  • National Natural Science Foundation of China (51608175)
  • Key Project of Science and Technology of the Education Department of Henan Province (17B610004)
  • Doctor Foundation of Henan Institute of Engineering (D2015020)

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CoChat. (2026). Citation check: Engineering MoS2 nanomesh with holes and lattice defects for highly active hydrogen evolution reaction. https://app.cochat.ai/papers/10.1016/j.apcatb.2018.05.080
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Li, Y., Yin, K., Wang, L., Lu, X., Zhang, Y., Liu, Y., Yan, D., Song, Y., & Luo, S. (2018). Engineering MoS2 nanomesh with holes and lattice defects for highly active hydrogen evolution reaction. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.05.080

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