The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Cobalt phthalocyanine coordinated to pyridine-functionalized carbon nanotubes with enhanced CO2 electroreduction
Abstract
Abstract Electrochemical reduction of CO2 is promising to utilize the intermittent renewable electricity and transform CO2 into value-added products, simultaneously. Herein, we designed a cobalt phthalocyanine-based catalyst supported on pyridine-functionalized carbon nanotubes (CoPc-py-CNT). This novel hybrid catalyst exhibited a high activity (TOFCO: 34.5 s−1 at −0.63 V vs. RHE) and selectivity (FECO > 98%) for electrochemical CO2 reduction. To the best of our knowledge, it is the best one among all reported molecular based electrocatalysts for CO2-to-CO conversion. Furthermore, structure characterizations (such as Raman and X-rays photoelectron spectroscopy), loading-dependent electrochemical analysis and mechanistic studies revealed that pyridine groups, through axial coordination with Co, not only functioned as physical promoters to improve the dispersion of cobalt phthalocyanine but also tuned the electronic structure of Co sites to increase the intrinsic turnover frequency.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Highly Efficient Electroreduction of CO2 to Methanol on Palladium–Copper Bimetallic Aerogels
Lu, L., Sun, X., Ma, J., Yang, D., Wu, H., Zhang, B., Zhang, J., & Han, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201808964 · Cited by 310
Cited by
Electrocatalytic reduction of carbon dioxide: opportunities with heterogeneous molecular catalysts
Sun, L., Reddu, V., Fisher, A. C., & Wang, X. (2020) · Energy & Environmental Science · doi:10.1039/c9ee03660a · Cited by 452
Boutin, E., Merakeb, L., Ma, B., Boudy, B., Wang, M., Bonin, J., Anxolabéhère-Mallart, E., & Robert, M. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00218f · Cited by 423
Metadata
- Authors
- Zhu, M., Chen, J., Guo, R., Xu, J., Fang, X., & Han, Y.-F.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2019-08
- Volume
- 251
- Pages
- 112-118
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2922092435
- Cited by
- 198
- References
- 4
- FWCI
- 5.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, M., Chen, J., Guo, R., Xu, J., Fang, X., & Han, Y.-F. (2019). Cobalt phthalocyanine coordinated to pyridine-functionalized carbon nanotubes with enhanced CO2 electroreduction. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2019.03.047
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