The DOI matches its Crossref record; 79 of the 79 references it cites were found in a registry or an index.
Sulfate saturated biosorbent-derived Co-S@NC nanoarchitecture as an efficient catalyst for peroxymonosulfate activation
Abstract
Abstract Using sulfate saturated bio-sorbent and cobalt(II) acetate as precursors, the homogeneous assembly of S-Co3O4 in nitrogen doped carbon martix (Co-S@NC) was obtained for the first time in an one-step pyrolysis. The reactions between peroxymonosulfate (PMS) and Co-S@NC for dinotefuran (DIN) decomposition were investigated. Co3O4 in Co@NC were primarily coordinated with the pyridinic N as catalytic sites. The adsorbed sulfate as S dopant was incorporated into the Co3O4 in carbon matrix due to the role of N as anchors, and the DIN decomposition of S-doped samples increased by 1.71 times as compared to the S-free sample (Co@NC). S incorporation can promote the formation of non-radical 1O2 and various radicals. In addition, DFT calculations indicated the enhanced electronic conductivity after S incorporation, which would facilitate the DIN decomposition in Co-S@NC/PMS system. This work enables the first insight into the role of adsorbed sulfate as effective S dopant for PMS activation.
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Cites
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Zhao, C., Shao, B., Yan, M., Liu, Z., Liang, Q., He, Q., Wu, T., Liu, Y., Pan, Y., Huang, J., et al. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2021.128829 · Cited by 518
Peng, L., Shang, Y., Gao, B., & Xu, X. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119484 · Cited by 478
Self-citationZhou, X., Zhao, Q., Wang, J., Chen, Z., & Chen, Z. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2020.128312 · Cited by 269
Zhou, X., Luo, M., Xie, C., Wang, H., Wang, J., Chen, Z., Xiao, J., & Chen, Z. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119605 · Cited by 253
Metadata
- Authors
- Du, W., Zhang, Q., Shang, Y., Wang, W., Li, Q., Yue, Q., Gao, B., & Xu, X.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2020-03
- Volume
- 262
- Pages
- 118302
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2980856288
- Cited by
- 432
- References
- 79
- FWCI
- 19.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- Du, W., Zhang, Q., Shang, Y., Wang, W., Li, Q., Yue, Q., Gao, B., & Xu, X. (2020). Sulfate saturated biosorbent-derived Co-S@NC nanoarchitecture as an efficient catalyst for peroxymonosulfate activation. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2019.118302
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