Low-temperature and high-voltage lithium-ion battery enabled by localized high-concentration carboxylate electrolytes

Feng, Tingting; Yang, Guozhu; Zhang, Shu; Xu, Ziqiang; Zhou, Haiping; Wu, Mengqiang

doi:10.1016/j.cej.2021.134138

Cited by 88Advanced Battery Materials and TechnologiesAdvancements in Battery MaterialsAdvanced Battery Technologies Research

Low-temperature and high-voltage lithium-ion battery enabled by localized high-concentration carboxylate electrolytes

Feng, Tingting, Yang, Guozhu, Zhang, Shu, Xu, Ziqiang, Zhou, Haiping, Wu, Mengqiang·2022·Chemical Engineering Journal

DOI 10.1016/j.cej.2021.134138

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This is the first attempt to use a localized high-concentration electrolyte for a high-voltage Li/LiNi0.5Mn1.5O4 system at low temperatures.
“It should be noticed that this is the first attempt to use LHCE for high-voltage Li/LNMO system at LTs.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [45]
When the salt concentration is 4 M, a Li/LiNi0.5Mn1.5O4 cell maintained 80.85% of its room-temperature specific discharge capacity at -50 °C.
“When the salt concentration is 4 M, the Li/LiNi 0.5 Mn 1.5 O 4 (LNMO) cell maintained 80.85% of its RT specific discharge capacity even at the LT of -50 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [45]
The electrochemical window of a localized high-concentration electrolyte containing LiBF4 in FEC/MA/TFME solvents is up to 5.4 V, and its ionic conductivity is 0.803-3.330 mS cm-1 in the temperature range from -50 to 25 °C.
“The electrochemical window of LHCE containing LiBF 4 in FEC/MA/TFME solvents is up to 5.4 V, and its ionic conductivity is measured to be 0.803-3.330mS cm -1 in the temperature range from -50 to 25 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [45]

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Solvation Deshielding Chemistry in γ‐Valerolactone‐Based Electrolytes Enables Fast Interfacial Charge Transfer Kinetics in Low‐Temperature Lithium‐Ion Capacitors
Xu, Y., Li, C., An, Y.-B., Li, Z., Ma, Y.-B., Sun, X.-Z., Wang, K., Zhang, X., & Ma, Y.-W. (2026) · Advanced Functional Materials · doi:10.1002/adfm.77840
Synergistic Influence of Electrolyte Additives on the Cycling Performance of Lithium-Ion Batteries under Extreme Fast Charging Condition
Dineshkumar, G., Backiyaleela, S. V., Jugović, D., Milović, M. D., & Stephan, A. (2026) · Energy · doi:10.1016/j.energy.2026.140237

Authors: Feng, T., Yang, G., Zhang, S., Xu, Z., Zhou, H., & Wu, M.
Affiliations: University of Electronic Science and Technology of China (CN)
Corresponding author: Feng, Tingting
Wu, Mengqiang
ORCID: Feng, Tingting
Yang, Guozhu
Xu, Ziqiang
Zhou, Haiping
Wu, Mengqiang
Venue: Chemical Engineering Journal
Publisher: Elsevier BV
Published: 2022-04
Volume: 433
Pages: 134138
ISSN: 1385-8947 (ISSN-L)
DOI: 10.1016/j.cej.2021.134138
OpenAlex: W4200563397
Cited by: 88
References: 0
Citations by year: 2026: 14 · 2025: 19 · 2024: 25 · 2023: 23 · 2022: 7
FWCI: 4.05
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
doi.org/10.15223/policy-017 (stm-asf)
doi.org/10.15223/policy-037 (stm-asf)
doi.org/10.15223/policy-012 (stm-asf)
doi.org/10.15223/policy-029 (stm-asf)
doi.org/10.15223/policy-004 (stm-asf)
Locations: Chemical Engineering Journal (publishedVersion)
Funders: Sichuan Province Science and Technology Support Program (2019ZDZX0029, 2020YFG0339, 2020ZHCG0035)
Science and Technology Department of Sichuan Province
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
Keywords: localized high-concentration electrolytes, lithium-ion batteries, high-voltage batteries, low-temperature operation, methyl acetate, LiNi0.5Mn1.5O4 cathode, cycling stability

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Low-temperature and high-voltage lithium-ion battery enabled by localized high-concentration carboxylate electrolytes

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