The DOI matches its Crossref record; 70 of the 70 references it cites were found in a registry or an index.
Electrochemical Synthesis of H2O2 by Two-Electron Water Oxidation Reaction
Open accessAbstract
Summary Hydrogen peroxide (H2O2) is a high-value green chemical oxidant widely used for industrial bleaching, chemical synthesis, and disinfection. Industrially, H2O2 is produced through the energy-intensive anthraquinone process and distributed to the point of use. There is a growing interest in electrochemically producing H2O2 onsite to mitigate transportation cost and safety concerns and leveraging renewable electricity. Most research has been dedicated to the two-electron oxygen reduction to produce H2O2. For the past decade, growing attention has been paid to the two-electron water oxidation reaction (2e-WOR) to produce H2O2. This review focuses on the research progress on 2e-WOR, including basic principles, catalyst development, and H2O2 detection. Computational approaches to study candidate materials for 2e-WOR are detailed, and various experimental reports on catalysts are summarized. Ulterior electrochemical factors that impact H2O2 production are discussed, along with device-level design. Finally, a holistic perspective on water oxidation reaction is offered, and open questions for future work are presented.
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Cites
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Metadata
- Authors
- Shi, X., Back, S., Gill, T. M., Siahrostami, S., & Zheng, X.
- Venue
- Chem
- Publisher
- Elsevier BV
- Published
- 2021-01
- Volume
- 7
- Issue
- 1
- Pages
- 38-63
- ISSN
- 2451-9294 (ISSN-L)
- OpenAlex
- W3093399657
- Cited by
- 429
- References
- 70
- FWCI
- 6.65
- Type
- journal article
- Language
- en
- Open access
- bronze
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