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The chromium isotopic composition of seawater and marine carbonates

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Bonnand, P., James, R.H., Parkinson, I.J., Connelly, D.P., Fairchild, I.J.·2013·Earth and Planetary Science Letters

DOI 10.1016/j.epsl.2013.09.001

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Abstract

Chromium isotopes are fractionated during redox reactions and have the potential to provide a record of changes in the oxygenation levels of the oceans in the geological past. However, Cr is a trace metal in seawater and its low concentrations make isotopic measurements challenging. Here we report the first determinations of δCr53 for seawater from open ocean (Argentine Basin) and coastal (Southampton Water) settings, using a double-spike technique. The total chromium concentration in seawater from Southampton Water is 1.85 nM, whereas the Cr content of Argentine Basin samples is 5.8–6.6 nM. The δCr53 value of seawater from the Argentine Basin is 0.491–0.556‰ in intermediate and deep waters, and varies between 0.412 and 0.664‰ in surface waters (<150 m). The δCr53 value of Southampton Water seawater is 1.505‰, which may reflect in situ reduction of Cr(VI) to Cr(III). All of our seawater samples have higher δCr53 than crustal and mantle silicates, and mass balance modelling demonstrates that river water must also be enriched in heavy Cr isotopes, indicating that Cr isotopes are fractionated during weathering and/or during transport to the oceans. We also show that the Cr isotopic composition of modern non-skeletal marine carbonates (0.640– 0.745‰) encompasses the range that we measure for Argentine Basin seawater. Thus, fractionation of Cr isotopes during precipitation of these marine carbonates is likely to be small (<0.2‰), and they have the potential to provide a record of the Cr isotopic composition of ancient seawater. Phanerozoic carbonates are also characterised by heavy δCr53 and a correlation between δCr53 and Ce/Ce⁎ suggests that the Cr and Ce cycles in the ocean are linked.

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Authors: Bonnand, P., James, R. H., Parkinson, I. J., Connelly, D. P., & Fairchild, I. J.
Affiliations: The Open University (GB)
National Oceanography Centre (GB)
University of Birmingham (GB)
Corresponding author: Bonnand, P.
ORCID: Bonnand, P.
James, R.H.
Parkinson, I.J.
Connelly, D.P.
Fairchild, I.J.
Venue: Earth and Planetary Science Letters
Publisher: Elsevier BV
Published: 2013-11
Volume: 382
Pages: 10-20
ISSN: 0012-821X (ISSN-L)
DOI: 10.1016/j.epsl.2013.09.001
OpenAlex: W2066760610
Cited by: 177
References: 84
Citations by year: 2026: 5 · 2025: 10 · 2024: 7 · 2023: 13 · 2022: 10 · 2021: 32 · 2020: 17 · 2019: 22 · 2018: 21 · 2017: 8 · 2016: 19 · 2015: 10 · 2014: 3
FWCI: 7.26
Type: journal article
Language: en
Open access: hybrid
doi.org
Licence: cc-by
www.elsevier.com/tdm/userlicense/1.0/ (tdm)
creativecommons.org/licenses/by/3.0/ (vor, 329 d)
Locations: Earth and Planetary Science Letters (publishedVersion, cc-by)
Bristol Research (University of Bristol) (publishedVersion)
NERC Open Research Archive (Natural Environment Research Council) (acceptedVersion)
ePrints Soton (University of Southampton) (acceptedVersion)
University of Birmingham Research Portal (University of Birmingham) (submittedVersion, cc-by)
Explore Bristol Research (submittedVersion)
Funders: Open University
Philip Leverhulme Prize (PLP/2006/0050)
RHJ
NERC (NE/H006443/1)
Topics: Physical Sciences › Earth and Planetary Sciences › Paleontology › Paleontology and Stratigraphy of Fossils
Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geochemistry and Elemental Analysis
Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geological and Geochemical Analysis
Keywords: chromium isotopes, seawater, marine carbonates, ocean oxygenation, hexavalent chromium reduction, weathering, mass balance model, Argentine Basin, Southampton Water

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The chromium isotopic composition of seawater and marine carbonates

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