Adsorption and desorption of SO 2 , NO and chlorobenzene on activated carbon
Open accessAbstract
Activated carbon (AC) is very effective for multi-pollutant removal; however, the complicated components in flue gas can influence each other's adsorption. A series of adsorption experiments for multicomponents, including SO2, NO, chlorobenzene and H2O, on AC were performed in a fixed-bed reactor. For single-component adsorption, the adsorption amount for chlorobenzene was larger than for SO2 and NO on the AC. In the multi-component atmosphere, the adsorption amount decreased by 27.6% for chlorobenzene and decreased by 95.6% for NO, whereas it increased by a factor of two for SO2, demonstrating that a complex atmosphere is unfavorable for chlorobenzene adsorption and inhibits NO adsorption. In contrast, it is very beneficial for SO2 adsorption. The temperature-programmed desorption (TPD) results indicated that the binding strength between the gas adsorbates and the AC follows the order of SO2>chlorobenzene > NO. The adsorption amount is independent of the binding strength. The presence of H2O enhanced the component effects, while it weakened the binding force between the gas adsorbates and the AC. AC oxygen functional groups were analyzed using TPD and X-ray photoelectron spectroscopy (XPS) measurements. The results reveal the reason why the chlorobenzene adsorption is less affected by the presence of other components. Lactone groups partly transform into carbonyl and quinone groups after chlorobenzene desorption. The chlorobenzene adsorption increases the number of C=O groups, which explains the positive effect of chlorobenzene on SO2 adsorption and the strong NO adsorption.
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The source of carbon determines the required pre-treatment step and the activation technique.
“the source of the carbon is also one of the key factors that determines the required pre-treatment step and the activation technique [37,47,70,125].”
From Biomass/Biochar carbon materials for CO2 capture and sequestration by cyclic adsorption processes: A review and prospects for future directions (2022) · cites this paper as [125]
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- Authors
- Li, Y., Guo, Y., Zhu, T., & Ding, S.
- Affiliations
- Chinese Academy of Sciences (CN)
- Corresponding author
- Zhu, Tingyu
- Venue
- Journal of Environmental Sciences
- Publisher
- Elsevier BV
- Published
- 2016-05
- Volume
- 43
- Issue
- 5
- Pages
- 128-135
- ISSN
- 1001-0742 (ISSN-L)
- OpenAlex
- W2235309997
- Cited by
- 71
- References
- 29
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- 4.45
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- journal article
- Language
- en
- Open access
- green
- ir.ipe.ac.cn
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- cc-by-nc-sa
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- Institute of Process Engineering, CAS Institutional Repository (submittedVersion, cc-by-nc-sa)
- Institute of Process Engineering, CAS Institutional Repository (submittedVersion)
- Funders
- National Natural Science Foundation of China (21177129, 21207132)
- Strategic Priority Research Program of the Chinese Academy of Sciences (XDB05050502)
- Topics
- Physical Sciences › Engineering › Mechanical Engineering › Industrial Gas Emission Control
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Keywords
- activated carbon, SO2 adsorption, NO adsorption, flue gas, multicomponent adsorption, adsorption inhibition, water vapor effect, oxygen-containing functional groups, lactone groups, temperature-programmed desorption, fixed-bed reactor, pollutant removal
- MeSH terms
- Adsorption, Air Pollutants, Charcoal, Chlorobenzenes, Models, Chemical, Nitrogen Oxides, Sulfur Dioxide
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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