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A review on 2D MoS2 cocatalysts in photocatalytic H2 production

Liang, Zizhan, Shen, Rongchen, Ng, Yun Hau, Zhang, Peng, Xiang, Quanjun, Li, Xin·2020·Journal of Materials Science & Technology

Abstract

Abstract Owing to their unique physicochemical, optical and electrical properties, two-dimensional (2D) MoS2 cocatalysts have been widely applied in designing and developing highly efficient composite photocatalysts for hydrogen generation under suitable light irradiation. In this review, we first elaborated on the fundamental aspects of 2D MoS2 cocatalysts to include the structural design principles, synthesis strategies, strengths and challenges. Subsequently, we thoroughly highlighted and discussed the modification strategies of 2D MoS2 H2-evolution cocatalysts, including doping heteroatoms (e.g. metals, non-metals, and co-doping), designing interfacial coupling morphologies, controlling the physical properties (e.g. thickness, size, structural defects or pores), exposing the reactive facets or edge sites, constructing cocatalyst heterojunctions, engineering the interfacial bonds and confinement effects. In the future, the forefront challenges in understanding and in precise controlling of the active sites at molecular level or atomic level should be carefully studied, while various potential mechanisms of photogenerated-electrons interactions should be proposed. The applications of MoS2 cocatalyst in the overall water splitting are also expected. This review may offer new inspiration for designing and constructing novel and efficient MoS2-based composite photocatalysts for highly efficient photocatalytic hydrogen evolution.

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Metadata

Authors
Liang, Z., Shen, R., Ng, Y. H., Zhang, P., Xiang, Q., & Li, X.
Venue
Journal of Materials Science & Technology
Publisher
Elsevier BV
Published
2020-11
Volume
56
Pages
89-121
ISSN
1005-0302 (ISSN-L)
OpenAlex
W3024548464
Cited by
438
References
12
FWCI
17.10
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: A review on 2D MoS2 cocatalysts in photocatalytic H2 production. https://app.cochat.ai/papers/10.1016/j.jmst.2020.04.032
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Liang, Z., Shen, R., Ng, Y. H., Zhang, P., Xiang, Q., & Li, X. (2020). A review on 2D MoS2 cocatalysts in photocatalytic H2 production. Journal of Materials Science & Technology. https://doi.org/10.1016/j.jmst.2020.04.032

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