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Cited by 396

The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.

Solid-Diffusion Synthesis of Single-Atom Catalysts Directly from Bulk Metal for Efficient CO2 Reduction

Open access
Zhao, Changming, Wang, Yu, Li, Zhijun, Chen, Wenxing, Xu, Qian, He, Dongsheng, Xi, Desheng, Zhang, Qinghua, Yuan, Tongwei, Qu, Yunteng, Yang, Jian, Zhou, Fangyao, Yang, Zhengkun, Wang, Xiaoqian, Wang, Jing, Luo, Jun, Li, Yafei, Duan, Haohong, Wu, Yuen, Li, Yadong·2019·Joule

Abstract

Summary Electroreduction of CO2 into value-added products is an effective approach to remit the environmental and energy issues. However, the development of an effective, accessible, and simple method for mass production of electrocatalyst is challenging. Herein, we demonstrate the solid-state diffusion between the N-doped carbon phase and bulk Ni metal can be utilized to synthesize hierarchical, self-supported, and atomistic catalyst. Strikingly, this hierarchical catalyst is programmable and scalable to meet the industrial demand and can be directly used as a binder-free electrode toward the CO2 electroreduction, delivering a state-of-the-art current density of 48.66 mA cm−2 at −1.0 V versus reversible hydrogen electrode (RHE) and high faradic efficiency of 97% to CO. The selectivity can be retained over 90% in a wide range of working potential of −0.7 to −1.2 V versus RHE. This solid-state diffusion strategy presents great potential to produce hierarchical and atomistic catalysts at industrial levels.

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Crossref · 10.1016/j.joule.2018.11.008

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Metadata

Authors
Zhao, C., Wang, Y., Li, Z., Chen, W., Xu, Q., He, D., Xi, D., Zhang, Q., Yuan, T., Qu, Y., Yang, J., Zhou, F., Yang, Z., Wang, X., Wang, J., Luo, J., Li, Y., Duan, H., Wu, Y., & Li, Y.
Venue
Joule
Publisher
Elsevier BV
Published
2019-02
Volume
3
Issue
2
Pages
584-594
ISSN
2542-4351 (ISSN-L)
OpenAlex
W2902358267
Cited by
396
References
38
FWCI
9.22
Type
journal article
Language
en
Open access
bronze
Licence
Funders
  • National Key R&D Program of China (2017YFA, 0208300, 0700100)
  • National Natural Science Foundation of China (21522107, 21671180, 21521091, U1463202, 21873050)

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CoChat. (2026). Citation check: Solid-Diffusion Synthesis of Single-Atom Catalysts Directly from Bulk Metal for Efficient CO2 Reduction. https://app.cochat.ai/papers/10.1016/j.joule.2018.11.008
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Zhao, C., Wang, Y., Li, Z., Chen, W., Xu, Q., He, D., Xi, D., Zhang, Q., Yuan, T., Qu, Y., Yang, J., Zhou, F., Yang, Z., Wang, X., Wang, J., Luo, J., Li, Y., Duan, H., Wu, Y., & Li, Y. (2019). Solid-Diffusion Synthesis of Single-Atom Catalysts Directly from Bulk Metal for Efficient CO2 Reduction. Joule. https://doi.org/10.1016/j.joule.2018.11.008

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.