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High-Efficiency Lithium-Metal Anode Enabled by Liquefied Gas Electrolytes
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“Usage of the stronger (compared to semifluorinated short alkanes) Li + coordinating nitriles such as acetonitrile, linear and cyclic ether cosolvents improved salt dissociation and solubility resulting in a substantial increase at LT.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [75]
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“The solvents also have extremely lowmelting points that render batteries operational below –60°C. Additives such as tetrahydrofuran (THF) (75) can be introduced to alter the Li+-solvation structure, which has been fully populated with CH3F molecules.”
BackgroundSelf-citationLiquid electrolyte: The nexus of practical lithium metal batteries
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Metadata
- Authors
- Yang, Y., Davies, D. M., Yin, Y., Borodin, O., Lee, J. Z., Fang, C., Olguin, M., Zhang, Y., Sablina, E. S., Wang, X., Rustomji, C. S., & Meng, Y. S.
- Affiliations
- University of California San Diego (US)
- DEVCOM Army Research Laboratory (US)
- Corresponding author
- Borodin, Oleg
- Rustomji, Cyrus S.
- Meng, Y. Shirley
- ORCID
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2019-08
- Volume
- 3
- Issue
- 8
- Pages
- 1986-2000
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2955217160
- Cited by
- 268
- References
- 40
- Citations by year
- 2026: 14 · 2025: 40 · 2024: 37 · 2023: 36 · 2022: 49 · 2021: 45 · 2020: 42 · 2019: 5
- FWCI
- 12.68
- Type
- journal article
- Language
- en
- Update notices
- erratum (2019-08-21)
- Open access
- bronze
- doi.org
- Licence
- Locations
- Joule (publishedVersion)
- eScholarship (California Digital Library) (submittedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- U.S. Department of Energy
- National Science Foundation
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Aqueous and Flow Batteries
- Keywords
- lithium metal anode, methyl fluoride, electrolyte solvation structure, lithium transference number, salt dissociation, dendrite suppression, Coulombic efficiency, lithium transport, rate capability, low-temperature cycling, solid-state batteries
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