The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Cu-Ag Tandem Catalysts for High-Rate CO2 Electrolysis toward Multicarbons
Open accessAbstract
Summary Tandem electrocatalysis decouples individual steps within a chemically complicated pathway via multicomponent catalyst design. Such a concept is attractive for CO2 electro-conversion to multicarbons (C2+), especially at high rates. Here, we show that a Cu-Ag tandem catalyst on a gas diffusion electrode (GDE) can enhance the C2+ production rate from CO2 through CO2 reduction to CO on Ag and subsequent carbon coupling on Cu. With added Ag, the C2+ partial current over a Cu surface increases from 37 to 160 mA/cm2 at −0.70 V versus reversible hydrogen electrode (RHE) in 1 M KOH with no mutual interference between the two metals. Moreover, the intrinsic C2H4 and C2H5OH activity in the tandem platform is significantly higher than Cu alone under either pure CO2 or CO atmosphere. Our results indicate that the CO-enriched local environment generated by Ag can enhance C2+ formation on Cu beyond CO2 or CO feeding, suggesting new mechanisms in a tandem three-phase environment.
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Combining theory and experiment in electrocatalysis: Insights into materials design
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CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
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What Should We Make with CO2 and How Can We Make It?
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Importance of Ag–Cu Biphasic Boundaries for Selective Electrochemical Reduction of CO2to Ethanol
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Wang, P., Yang, H., Tang, C., Wu, Y., Zheng, Y., Cheng, T., Davey, K., Huang, X., & Qiao, S.-Z. (2022) · Nature Communications · doi:10.1038/s41467-022-31427-9 · Cited by 574
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Li, L., Li, X., Sun, Y., & Xie, Y. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00893e · Cited by 448
Engineering Cu(I)/Cu(0) interfaces for efficient ethanol production from CO2 electroreduction
Cai, R., Sun, M., Yang, F., Ju, M., Chen, Y., Gu, M. D., Huang, B., & Yang, S. (2024) · Chem · doi:10.1016/j.chempr.2023.08.027 · Cited by 142
Metadata
- Authors
- Chen, C., Li, Y., Yu, S., Louisia, S., Jin, J., Li, M., Ross, M. B., & Yang, P.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2020-08
- Volume
- 4
- Issue
- 8
- Pages
- 1688-1699
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W3048431271
- Cited by
- 502
- References
- 10
- FWCI
- 10.89
- Type
- journal article
- Language
- en
- Open access
- bronze
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