PEMFC electrode preparation: Influence of the solvent composition and evaporation rate on the catalytic layer microstructure
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The dielectric constant of the solvent affects catalyst-ionomer aggregation size; excessively high or low dielectric constant leads to significant ink agglomeration.
“First, the dielectric constant of the solvent affects the catalyst-ionomer aggregation size: when excessively high or low, the dielectric constant leads to significant ink agglomeration.”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [175]
A solvent with a moderate dielectric constant is helpful in improving ink stability.
“A solvent with a moderate dielectric constant would be helpful in improving the ink stability [174,175].”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [175]
Cites
Passalacqua, E., Lufrano, F., Squadrito, G., Patti, A., & Giorgi, L. (2001) · Electrochimica Acta · doi:10.1016/s0013-4686(00)00679-4 · Cited by 440 · see citing works
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Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly
Mo, S., Du, L., Huang, Z., Chen, J., Zhou, Y., Wu, P., Meng, L., Wang, N., Xing, L., Zhao, M., et al. (2023) · Electrochemical Energy Reviews · doi:10.1007/s41918-023-00190-w · Cited by 277 · see citing works
“A solvent with a moderate dielectric constant would be helpful in improving the ink stability [174, 175].”
Ngo, T. T., Yu, T. L., & Lin, H.-L. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2012.10.055 · Cited by 231 · see citing works
The Controllable Design of Catalyst Inks to Enhance PEMFC Performance: A Review
Guo, Y., Pan, F., Chen, W., Ding, Z., Yang, D., Li, B., Ming, P., & Zhang, C. (2021) · Electrochemical Energy Reviews · doi:10.1007/s41918-020-00083-2 · Cited by 175 · see citing works
Takahashi, S., Mashio, T., Horibe, N., Akizuki, K., & Ohma, A. (2015) · ChemElectroChem · doi:10.1002/celc.201500131 · Cited by 143 · see citing works
Inherent Acidity of Perfluorosulfonic Acid Ionomer Dispersions and Implications for Ink Aggregation
Berlinger, S. A., McCloskey, B. D., & Weber, A. Z. (2018) · The Journal of Physical Chemistry B · doi:10.1021/acs.jpcb.8b06493 · Cited by 122 · see citing works
Kim, T.-H., Yi, J.-Y., Jung, C.-Y., Jeong, E., & Yi, S.-C. (2017) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2016.12.015 · Cited by 127 · see citing works
Effect of dispersion solvent in catalyst ink on proton exchange membrane fuel cell performance
Huang, D.-C., Yu, P.-J., Liu, F.-J., Huang, S.-L., Hsueh, K.-L., Chen, Y.-C., Wu, C.-H., Chang, W.-C., & Tsau, F.-H. (2011) · International Journal of Electrochemical Science · doi:10.1016/s1452-3981(23)18202-2 · Cited by 93 · see citing works
Ngo, T. T., Yu, T. L., & Lin, H.-L. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2013.03.055 · Cited by 92 · see citing works
Impact of Catalyst Ink Dispersing Solvent on PEM Fuel Cell Performance and Durability
Lei, C., Yang, F., Macauley, N., Spinetta, M., Purdy, G., Jankovic, J., Cullen, D. A., More, K. L., Kim, Y. S., & Xu, H. (2021) · Journal of The Electrochemical Society · doi:10.1149/1945-7111/abf2b0 · Cited by 93 · see citing works
Gravure coating for roll-to-roll manufacturing of proton-exchange-membrane fuel cell catalyst layers
Mauger, S. A., Neyerlin, K. C., Yang-Neyerlin, A. C., More, K. L., & Ulsh, M. (2018) · Journal of The Electrochemical Society · doi:10.1149/2.0091813jes · Cited by 81 · see citing works
Molecular Dynamics Study of Ionomer Adsorption at a Carbon Surface in Catalyst Ink
Mashio, T., Ohma, A., & Tokumasu, T. (2016) · Electrochimica Acta · doi:10.1016/j.electacta.2016.04.004 · Cited by 84 · see citing works
Wang, G., Zou, L., Huang, Q., Zou, Z., & Yang, H. (2019) · Journal of Materials Chemistry A · doi:10.1039/c8ta12382a · Cited by 81 · see citing works
Dispersion-Solvent Control of Ionomer Aggregation in a Polymer Electrolyte Membrane Fuel Cell
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Effect of catalytic ink on sub-freezing endurance of PEMFCs
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- Authors
- Fernández, R., Ferreira-Aparicio, P., & Daza, L.
- Affiliations
- Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas (ES)
- Instituto de Catálisis y Petroleoquímica (ES)
- Corresponding author
- Ferreira-Aparicio, P.
- Venue
- Journal of Power Sources
- Publisher
- Elsevier BV
- Published
- 2005-10
- Volume
- 151
- Pages
- 18-24
- ISSN
- 0378-7753 (ISSN-L)
- OpenAlex
- W2004816004
- Cited by
- 120
- References
- 1
- Citations by year
- 2026: 6 · 2025: 6 · 2024: 4 · 2023: 6 · 2022: 9 · 2021: 10 · 2020: 5 · 2019: 6 · 2018: 6 · 2017: 1 · 2016: 6 · 2015: 3 · 2014: 3 · 2013: 7 · 2012: 3
- FWCI
- 6.97
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Power Sources (publishedVersion)
- Funders
- Universidad Nacional de Educación a Distancia
- Ministerio de Educación, Cultura y Deporte (MAT2002-03125)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Advancements in Solid Oxide Fuel Cells
- Keywords
- proton exchange membrane fuel cells, solvent composition, solvent evaporation rate, Nafion ionomer, solvent viscosity, solvent dielectric constant, electrode performance
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