The DOI matches its Crossref record; 23 of the 23 references it cites were found in a registry or an index.
Tuning Zn2+ coordination environment to suppress dendrite formation for high-performance Zn-ion batteries
Abstract
Abstract The short-circuit issue induced by Zn dendrite growth restricts the commercialization of rechargeable aqueous Zn-ion batteries (ZIBs). Herein, ethylene glycol (EG), a representative of dihydric alcohols, is applied in the aqueous electrolyte to inhibit the detrimental dendrite growth on Zn anode. Our work demonstrates a uniform Zn plating/stripping in H2O/EG hybrid electrolyte with cycling lifespan of up to 2668 h at 0.5 mA cm−2, which is made possible by the substitution of EG for H2O in the solvation sheath of Zn2+ ions. Such a change in the coordination environment of Zn2+ gives rise to decreased diffusivity of the ions and increased over-potential for nucleation, further resulting in even deposition morphology rather than large-scale dendrites. Side reactions are also circumvented by the formation of hydrogen bonds. All these aspects work in synergy to promote the cyclability of the assembled full battery. The low-cost aqueous electrolyte identified in this work opens up new opportunities for manipulating the coordination environments of Zn2+ ions and optimizing the Zn deposition morphology during the design of high-performance ZIBs.
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Cites
Highly reversible zinc metal anode for aqueous batteries
Wang, F., Borodin, O., Gao, T., Fan, X., Sun, W., Han, F., Faraone, A., Dura, J. A., Xu, K., & Wang, C. (2018) · Nature Materials · doi:10.1038/s41563-018-0063-z · Cited by 3,305
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Nanoscale Nucleation and Growth of Electrodeposited Lithium Metal
Pei, A., Zheng, G., Shi, F., Li, Y., & Cui, Y. (2017) · Nano Letters · doi:10.1021/acs.nanolett.6b04755 · Cited by 1,726
Self-citationAdvanced rechargeable zinc-based batteries: Recent progress and future perspectives
Li, H., Ma, L., Han, C., Wang, Z., Liu, Z., Tang, Z., & Zhi, C. (2019) · Nano Energy · doi:10.1016/j.nanoen.2019.05.059 · Cited by 1,167
Self-citationYang, H., Chang, Z., Qiao, Y., Deng, H., Mu, X., He, P., & Zhou, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202001844 · Cited by 845
Aqueous vs. nonaqueous Zn-ion batteries: consequences of the desolvation penalty at the interface
Kundu, D., Hosseini Vajargah, S., Wan, L., Adams, B., Prendergast, D., & Nazar, L. F. (2018) · Energy & Environmental Science · doi:10.1039/c8ee00378e · Cited by 833
A ZnCl2 water-in-salt electrolyte for a reversible Zn metal anode
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A flexible rechargeable aqueous zinc manganese-dioxide battery working at −20 °C
Mo, F., Liang, G., Meng, Q., Liu, Z., Li, H., Fan, J., & Zhi, C. (2019) · Energy & Environmental Science · doi:10.1039/c8ee02892c · Cited by 687
Cited by
Recent Progress on Zn Anodes for Advanced Aqueous Zinc‐Ion Batteries
Nie, C., Wang, G., Wang, D., Wang, M., Gao, X., Bai, Z., Wang, N., Yang, J., Xing, Z., & Dou, S. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300606 · Cited by 561
Li, M., Li, Z., Wang, X., Meng, J., Liu, X., Wu, B., Han, C., & Mai, L. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00030f · Cited by 559
Non-concentrated aqueous electrolytes with organic solvent additives for stable zinc batteries
Dong, Y., Miao, L., Ma, G., Di, S., Wang, Y., Wang, L., Xu, J., & Zhang, N. (2021) · Chemical Science · doi:10.1039/d0sc06734b · Cited by 489
Self-citationLiu, Z., Wang, R., Ma, Q., Wan, J., Zhang, S., Zhang, L., Li, H., Luo, Q., Wu, J., Zhou, T., et al. (2024) · Advanced Functional Materials · doi:10.1002/adfm.202214538 · Cited by 394
Designing Electrolyte Structure to Suppress Hydrogen Evolution Reaction in Aqueous Batteries
Nian, Q., Zhang, X., Feng, Y., Liu, S., Sun, T., Zheng, S., Ren, X., Tao, Z., Zhang, D., & Chen, J. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.1c00833 · Cited by 303
Metadata
- Authors
- Qin, R., Wang, Y., Zhang, M., Wang, Y., Ding, S., Song, A., Yi, H., Yang, L., Song, Y., Cui, Y., Liu, J., Wang, Z., Li, S., Zhao, Q., & Pan, F.
- Venue
- Nano Energy
- Publisher
- Elsevier BV
- Published
- 2021-02
- Volume
- 80
- Pages
- 105478
- ISSN
- 2211-2855 (ISSN-L)
- OpenAlex
- W3092749977
- Cited by
- 585
- References
- 23
- FWCI
- 25.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Qin, R., Wang, Y., Zhang, M., Wang, Y., Ding, S., Song, A., Yi, H., Yang, L., Song, Y., Cui, Y., Liu, J., Wang, Z., Li, S., Zhao, Q., & Pan, F. (2021). Tuning Zn2+ coordination environment to suppress dendrite formation for high-performance Zn-ion batteries. Nano Energy. https://doi.org/10.1016/j.nanoen.2020.105478
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