The DOI matches its Crossref record; 235 of the 237 references it cites were found in a registry or an index.
Fate and transport of per- and polyfluoroalkyl substances (PFASs) in the vadose zone
Open accessAbstract
Per- and polyfluoroalkyl substances (PFASs) are a heterogeneous group of persistent organic pollutants that have been detected in various environmental compartments around the globe. Emerging research has revealed the preferential accumulation of PFASs in shallow soil horizons, particularly at sites impacted by firefighting activities, agricultural applications, and atmospheric deposition. Once in the vadose zone, PFASs can sorb to soil, accumulate at interfaces, become volatilized, be taken up in biota, or leach to the underlying aquifer. At the same time, polyfluorinated precursor species may transform into highly recalcitrant perfluoroalkyl acids, changing their chemical identity and thus transport behavior along the way. In this review, we critically discuss the current state of the knowledge and aim to interconnect the complex processes that control the fate and transport of PFASs in the vadose zone. Furthermore, we identify key challenges and future research needs. Consequently, this review may serve as an interdisciplinary guide for the risk assessment and management of PFAS-contaminated sites.
Overview
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
In the citing paper
“Briefly, PFAS and their precursors can be removed by adsorption to soil minerals, air-water interfaces, and microbial biomass or roots, translocated into plants, and degraded or transformed by soil microorganisms.”
From Perfluoroalkyl acids on suspended particles: Significant transport pathways in surface runoff, surface waters, and subsurface soils (2021) · cites this paper as Sharifan et al., 2021
In the citing paper
“Short-chain PFASs (CF2,3 < 6) are relatively more mobile and thus more susceptible to leaching compared to the longer-chain homologues.14,15”
From Sources and Pathways of PFAS Occurrence in Water Sources: Relative Contribution of Land-Applied Biosolids in an Agricultural Dominated Watershed (2025) · cites this paper as [15]
Citations
Cites
1 retracted
Items 201–235 of 235
Jin, B., Mallula, S., Golovko, S. A., Golovko, M. Y., & Xiao, F. (2020) · Environmental Science & Technology · doi:10.1021/acs.est.0c01644 · Cited by 54
Nobels, I., Dardenne, F., Coen, W. D., & Blust, R. (2010) · Toxicology in Vitro · doi:10.1016/j.tiv.2010.07.002 · Cited by 52
Fast Generation of Perfluoroalkyl Acids from Polyfluoroalkyl Amine Oxides in Aerobic Soils
Chen, H., Liu, M., Munoz, G., Duy, S. V., Sauvé, S., Yao, Y., Sun, H., & Liu, J. (2020) · Environmental Science & Technology Letters · doi:10.1021/acs.estlett.0c00543 · Cited by 50
Self-citationSorption of perfluoroalkyl substances in sewage sludge
Milinovic, J., Lacorte, S., Rigol, A., & Vidal, M. (2016) · Environmental Science and Pollution Research · doi:10.1007/s11356-015-6019-9 · Cited by 50
Blotevogel, J., Giraud, R. J., & Borch, T. (2017) · Chemical Engineering Journal · doi:10.1016/j.cej.2017.10.131 · Cited by 49
Self-citationDetermination of Water-Oil Interfacial Area during 3-Phase Gravity Drainage in Porous Media
Schaefer, C. E., DiCarlo, D. A., & Blunt, M. J. (2000) · Journal of Colloid and Interface Science · doi:10.1006/jcis.1999.6604 · Cited by 47
Self-citationYi, L., Peng, Q., Liu, D., Zhou, L., Tang, C., Zhou, Y., & Chai, L. (2018) · Environmental Technology · doi:10.1080/09593330.2018.1466918 · Cited by 47
Gribble, M. O., Bartell, S. M., Kannan, K., Wu, Q., Fair, P. A., & Kamen, D. L. (2015) · Environmental Research · doi:10.1016/j.envres.2015.03.012 · Cited by 43
Thermodynamic Considerations for Dehalogenation
Jan, D. (2005) · Kluwer Academic Publishers eBooks · doi:10.1007/0-306-48011-5_4 · Cited by 42
Londono, N., Donovan, A. R., Shi, H., Geisler, M. J., & Liang, Y. (2017) · Nanotoxicology · doi:10.1080/17435390.2017.1401141 · Cited by 42
Self-citationDasu, K., Lee, L. S., Turco, R. F., & Nies, L. F. (2013) · Chemosphere · doi:10.1016/j.chemosphere.2012.11.076 · Cited by 42
Soil Microbial Communities as Indicators of Soil Health
Kennedy, A. C., & Stubbs, T. L. (2006) · Annals of Arid Zone · doi:10.56093/aaz.v45i3 · Cited by 41
Bacterial community in a freshwater pond responding to the presence of perfluorooctanoic acid (PFOA)
Zhang, D., Zhang, W., & Liang, Y. (2019) · Environmental Technology · doi:10.1080/09593330.2019.1616828 · Cited by 39
Self-citationSale, T. C., Gallo, S., Askarani, K. K., Irianni-Renno, M., Lyverse, M., Hopkins, H., Blotevogel, J., & Burge, S. R. (2020) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2020.124403 · Cited by 38
Self-citationMuschket, M., Keltsch, N., Paschke, H., Reemtsma, T., & Berger, U. (2020) · Journal of Chromatography A · doi:10.1016/j.chroma.2020.461271 · Cited by 34
Aerobic Soil Biotransformation of 6:2 Fluorotelomer Iodide
Ruan, T., Szostek, B., Folsom, P. W., Wolstenholme, B. W., Liu, R., Liu, J., Jiang, G., Wang, N., & Buck, R. C. (2013) · Environmental Science & Technology · doi:10.1021/es4018128 · Cited by 30
Self-citationIn-Situ Molecular-Level Elucidation of Organofluorine Binding Sites in a Whole Peat Soil
Longstaffe, J. G., Courtier‐Murias, D., Soong, R., Simpson, M. J., Maas, W. E., Fey, M., Hutchins, H., Krishnamurthy, S., Struppe, J. O., Alaee, M., et al. (2012) · Environmental Science & Technology · doi:10.1021/es3026769 · Cited by 29
Comment on “Uptake of Poly- and Perfluoroalkyl Substances at the Air–Water Interface”
Arshadi, M., Costanza, J., Abriola, L. M., & Pennell, K. D. (2020) · Environmental Science & Technology · doi:10.1021/acs.est.0c01838 · Cited by 29
Schaefer, C. E., Nguyen, D., & Field, J. A. (2020) · Environmental Science & Technology · doi:10.1021/acs.est.0c02488 · Cited by 29
Self-citationSharifan, H., Wang, X., & Ma, X. (2019) · International Journal of Phytoremediation · doi:10.1080/15226514.2019.1658713 · Cited by 26
Self-citationCryogenic Core Collection (C 3 ) from Unconsolidated Subsurface Media
Kiaalhosseini, S., Johnson, R. L., Rogers, R. C., Irianni-Renno, M., Lyverse, M., & Sale, T. C. (2016) · Groundwater Monitoring & Remediation · doi:10.1111/gwmr.12186 · Cited by 22
Dasu, K., Royer, L. A., Liu, J., & Lee, L. (2010) · Chemosphere · doi:10.1016/j.chemosphere.2010.07.068 · Cited by 21
Self-citationLondono, N., Donovan, A. R., Shi, H., Geisler, M. J., & Liang, Y. (2019) · Chemosphere · doi:10.1016/j.chemosphere.2019.05.110 · Cited by 21
Self-citationPerfluoroalkyl Substances in the Environment
Kempisty, D. M., Xing, Y., & Racz, L. (2018) · CRC Press eBooks · doi:10.1201/9780429487125 · Cited by 20
Comment on “Biodegradation of perfluorooctanesulfonate (PFOS) as an emerging contaminant”
Avendaño, S. M., Zhong, G., & Liu, J. (2015) · Chemosphere · doi:10.1016/j.chemosphere.2015.03.022 · Cited by 19
Self-citationAssessing and Managing Chemicals under TSCA
Ocspp, & Oppt (2013) · Cited by 19
Dasu, K., & Lee, L. (2015) · Chemosphere · doi:10.1016/j.chemosphere.2015.11.021 · Cited by 15
Use and Potential Impacts of AFFF Containing PFASs at Airports
Thalheimer, A. H., McConney, L. B., Kalinovich, I. K., Pigott, A. V., Franz, J. D., Holbert, H. T., Mericas, D., Puchacz, Z. J., & University of Washington (2017) · Transportation Research Board eBooks · doi:10.17226/24800 · Cited by 13
Fluorosurfactants in Firefighting Foams
Korzeniowski, S. H., Buck, R. C., Kempisty, D. M., & Pabon, M. (2018) · CRC Press eBooks · doi:10.1201/9780429487125-1 · Cited by 13
Thermodynamic considerations for dehalogenation
Dolfing, J. (2003) · Socio-Environmental Systems Modeling · doi:10.25405/ncl.34583112 · Cited by 11
Sharifan, H. (2020) · Environmental Monitoring and Assessment · doi:10.1007/s10661-020-08309-y · Cited by 8
Self-citationSung, M., & Chen, B.-H. (2011) · Journal of Contaminant Hydrology · doi:10.1016/j.jconhyd.2011.09.001 · Cited by 6
Correlation of physico-chemical parameters with toxicity of metal ions to plants
Enache, M., Palit, P., Dearden, J. C., & Lepp, N. W. (2000) · Pest Management Science · doi:10.1002/1526-4998(200009)56:9 · Cited by 5
Sharifan, H. (2017) · Environmental Pollution · doi:10.1016/j.envpol.2017.06.018 · Cited by 1
Self-citationSpridning av högfluorerade ämnen i mark från Stockholm Arlanda Airport
Rosenqvist, L., Vestergren, R., Westberg, E., Eliaeson, K., Liljeberg, M., Strandberg, J., Rahmberg, M., & Norström, K. (2017) · KTH Publication Database DiVA (KTH Royal Institute of Technology) · Cited by 1
Flagged first, then by citations
2 of the 237 references couldn’t be matched to a known paper.
Research works printed but not linked: 2
- Krepich, 2019, 15, 30
- Luo, 2018, 539, 241
Cited by
Sorted by citations
Kurwadkar, S., Dane, J., Kanel, S. R., Nadagouda, M. N., Cawdrey, R. W., Ambade, B., Struckhoff, G. C., & Wilkin, R. (2022) · Science of The Total Environment · doi:10.1016/j.scitotenv.2021.151003 · Cited by 937
PFAS Molecules: A Major Concern for the Human Health and the Environment
Panieri, E., Baralic, K., Djukic-Cosic, D., Buha Djordjevic, A., & Saso, L. (2022) · Toxics · doi:10.3390/toxics10020044 · Cited by 651
Wang, D., Xiao, F., Xiao, F., Chen, J., Park, C. M., Park, C. M., Flury, M., & Flury, M. (2022) · Reviews of Geophysics · doi:10.1029/2021rg000765 · Cited by 294
Self-citationMenger, R. F., Funk, E., Henry, C. S., & Borch, T. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2021.129133 · Cited by 224
Updated review on emerging technologies for PFAS contaminated water treatment
Yadav, S., Ibrar, I., Al-Juboori, R. A., Singh, L., Ganbat, N., Kazwini, T., Karbassiyazdi, E., Samal, A. K., Subbiah, S., & Altaee, A. (2022) · Process Safety and Environmental Protection · doi:10.1016/j.cherd.2022.04.009 · Cited by 184
Metadata
- Authors
- Sharifan, H., Bagheri, M., Wang, D., Burken, J. G., Higgins, C. P., Liang, Y., Liu, J., Schaefer, C. E., & Blotevogel, J.
- Affiliations
- Colorado State University (US)
- Missouri University of Science and Technology (US)
- McGill University (CA)
- Colorado School of Mines (US)
- University at Albany, State University of New York (US)
- CDM Smith (United States) (US)
- Corresponding author
- Blotevogel, Jens
- ORCID
- Venue
- Science of The Total Environment
- Publisher
- Elsevier BV
- Published
- 2021-06
- Volume
- 771
- Pages
- 145427
- ISSN
- 0048-9697 (ISSN-L)
- OpenAlex
- W3124974648
- Cited by
- 180
- References
- 237
- Citations by year
- 2026: 34 · 2025: 39 · 2024: 38 · 2023: 18 · 2022: 36 · 2021: 15
- FWCI
- 1.98
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- www.elsevier.com/tdm/userlicense/1.0/ (tdm)
- www.elsevier.com/legal/tdmrep-license (tdm)
- www.elsevier.com/open-access/userlicense/1.0/ (am, 249 d)
- doi.org/10.15223/policy-017 (stm-asf)
- doi.org/10.15223/policy-037 (stm-asf)
- doi.org/10.15223/policy-012 (stm-asf)
- doi.org/10.15223/policy-029 (stm-asf)
- doi.org/10.15223/policy-004 (stm-asf)
- Locations
- The Science of The Total Environment (acceptedVersion)
- PubMed (publishedVersion)
- Funders
- Natural Sciences and Engineering Research Council of Canada
- National Science Foundation
- Strategic Environmental Research and Development Program
- University at Albany
- Topics
- Physical Sciences › Environmental Science › Environmental Chemistry › Per- and polyfluoroalkyl substances research
- Physical Sciences › Chemistry › Organic Chemistry › Fluorine in Organic Chemistry
- Physical Sciences › Environmental Science › Pollution › Pesticide and Herbicide Environmental Studies
- Keywords
- per- and polyfluoroalkyl substances, PFAS fate and transport, vadose zone, soil sorption, volatilization, perfluoroalkyl acids, atmospheric deposition
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review