Cited by 238Adsorption and biosorption for pollutant removalUrban Stormwater Management SolutionsHeavy Metal Pollution Remediation

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Simultaneous removal of As, Cd, Cr, Cu, Ni and Zn from stormwater: Experimental comparison of 11 different sorbents

Genç-Fuhrman, Hülya, Mikkelsen, Peter S., Ledin, Anna·2007·Water Research

DOI 10.1016/j.watres.2006.10.024

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Abstract

The potential of using alumina, activated bauxsol-coated sand (ABCS), bark, bauxsol-coated sand (BCS), fly ash (FA), granulated activated carbon (GAC), granulated ferric hydroxide (GFH), iron oxide-coated sand (IOCS), natural zeolite (NZ), sand, and spinel (MgAl(2)O(4)) as sorbents for removing heavy metals from stormwater are investigated in the present study. The ability of the sorbents to remove a mixture of As, Cd, Cr, Cu, Ni and Zn from synthetic stormwater samples were evaluated in batch tests at a starting pH of 6.5. The metal speciation and saturation data is obtained using the PHREEQ-C geochemical model and used to elucidate the sorption data. It is found that BCS, FA, and spinel have significantly higher affinity towards heavy metals mainly present as cationic or non-charged species (i.e. Cd, Cu, Ni and Zn) compared to those present as anionic species (i.e. As and Cr). However, IOCS, NZ and sand have higher affinity towards As and Cr, while alumina has equally high affinity to all tested heavy metals. The Freundlich isotherm model is found to fit the data in many cases, but ill fitted results are also observed, especially for FA, BCS and GAC, possibly due to leaching of some metals from the sorbents (i.e. for FA) and oversaturated conditions making precipitation the dominant removal mechanism over sorption in batches with high heavy metal concentrations and pH. Calculated sorption constants (i.e. K(d)) are used to compare the overall heavy metal removal efficiency o…

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Authors: Genç-Fuhrman, H., Mikkelsen, P. S., & Ledin, A.
Affiliations: Technical University of Denmark (DK)
Corresponding author: Genç-Fuhrman, Hülya
ORCID: Mikkelsen, Peter S.
Venue: Water Research
Publisher: Elsevier BV
Published: 2007-02
Volume: 41
Issue: 3
Pages: 591-602
ISSN: 0043-1354 (ISSN-L)
DOI: 10.1016/j.watres.2006.10.024
OpenAlex: W2036209727
Cited by: 238
References: 33
Citations by year: 2026: 2 · 2025: 1 · 2024: 5 · 2023: 7 · 2022: 8 · 2021: 7 · 2020: 10 · 2019: 10 · 2018: 20 · 2017: 7 · 2016: 16 · 2015: 23 · 2014: 22 · 2013: 17 · 2012: 15
FWCI: 14.63
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Water Research (publishedVersion)
PubMed (publishedVersion)
Technical University of Denmark, DTU Orbit (Technical University of Denmark, DTU) (submittedVersion)
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
Physical Sciences › Environmental Science › Environmental Engineering › Urban Stormwater Management Solutions
Physical Sciences › Environmental Science › Water Science and Technology › Heavy Metal Pollution Remediation
Keywords: stormwater treatment, heavy metal removal, sorbents, arsenic, cadmium, chromium, copper, nickel, zinc, fly ash, granular activated carbon, spinel, natural zeolite, iron oxide-coated sand, alumina, Freundlich isotherm, metal speciation, sorption constants, metal leaching, precipitation chemistry
MeSH terms: Adsorption, Cadmium, Chromium, Copper, Hydrogen-Ion Concentration, Nickel, Water Pollutants, Chemical, Zinc, Water Purification, Metals, Heavy

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Simultaneous removal of As, Cd, Cr, Cu, Ni and Zn from stormwater: Experimental comparison of 11 different sorbents

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