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Bulk-Type All Solid-State Batteries with 5 V Class LiNi0.5Mn1.5O4 Cathode and Li10GeP2S12 Solid Electrolyte
Abstract
All solid-state batteries are of key importance in the development of next-generation energy storage devices with high energy density. Herein, we report the fabrication and operation of bulk-type 5 V-class all solid-state batteries consisting of LiNi 0.5 Mn 1.5 O 4 cathode, Li 10 GeP 2 S 12 solid-electrolyte, and Li metal anode. The 1st discharge capacity is about 80 mAh g –1 with an average voltage of 4.3 V. The discharge capacity gradually decreases during the subsequent cycles. X-ray diffraction and electrochemical impedance spectroscopy measurements reveal that the capacity fading results from the growth of a resistive interfacial layer on the cathode composite. The development of suitable conductive additive and sulfide solid electrolyte materials is essential for the development of high-voltage all solid-state batteries.
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Cited by
A solid future for battery development
Janek, J., & Zeier, W. G. (2016) · Nature Energy · doi:10.1038/nenergy.2016.141 · Cited by 3,979
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Koerver, R., Aygün, I., Leichtweiß, T., Dietrich, C., Zhang, W., Binder, J. O., Hartmann, P., Zeier, W. G., & Janek, J. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b00931 · Cited by 1,020
Zhang, W., Weber, D. A., Weigand, H., Arlt, T., Manke, I., Schröder, D., Koerver, R., Leichtweiss, T., Hartmann, P., Zeier, W. G., et al. (2017) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.7b01137 · Cited by 538
Li, W., Dolocan, A., Oh, P., Celio, H., Park, S., Cho, J., & Manthiram, A. (2017) · Nature Communications · doi:10.1038/ncomms14589 · Cited by 466
Metadata
- Authors
- Oh, G., Hirayama, M., Kwon, O., Suzuki, K., & Kanno, R.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-04-12
- Volume
- 28
- Issue
- 8
- Pages
- 2634-2640
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2329970688
- Cited by
- 278
- References
- 0
- FWCI
- 13.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- Oh, G., Hirayama, M., Kwon, O., Suzuki, K., & Kanno, R. (2016). Bulk-Type All Solid-State Batteries with 5 V Class LiNi0.5Mn1.5O4 Cathode and Li10GeP2S12 Solid Electrolyte. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.5b04940
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