Cited by 2,406Carbon Dioxide Capture TechnologiesCO2 Sequestration and Geologic InteractionsCarbon dioxide utilization in catalysis

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Direct Capture of CO2 from Ambient Air

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Sanz-Pérez, Eloy S., Murdock, Christopher R., Didas, Stephanie A., Jones, Christopher W.·2016·Chemical Reviews

DOI 10.1021/acs.chemrev.6b00173

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Abstract

The increase in the global atmospheric CO2 concentration resulting from over a century of combustion of fossil fuels has been associated with significant global climate change. With the global population increase driving continued increases in fossil fuel use, humanity’s primary reliance on fossil energy for the next several decades is assured. Traditional modes of carbon capture such as precombustion and postcombustion CO2 capture from large point sources can help slow the rate of increase of the atmospheric CO2 concentration, but only the direct removal of CO2 from the air, or “direct air capture” (DAC), can actually reduce the global atmospheric CO2 concentration. The past decade has seen a steep rise in the use of chemical sorbents that are cycled through sorption and desorption cycles for CO2 removal from ultradilute gases such as air. This Review provides a historical overview of the field of DAC, along with an exhaustive description of the use of chemical sorbents targeted at this application. Solvents and solid sorbents that interact strongly with CO2 are described, including basic solvents, supported amine and ammonium materials, and metal–organic frameworks (MOFs), as the primary classes of chemical sorbents. Hypothetical processes for the deployment of such sorbents are discussed, as well as the limited array of technoeconomic analyses published on DAC. Overall, it is concluded that there are many new materials that could play a role in emerging DAC technologies. However, these materials need to be further investigated and developed with a practical sorbent–air contacting process in mind if society is to make rapid progress in deploying DAC as a means of mitigating climate change.

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Self-citation

Authors: Sanz-Pérez, E. S., Murdock, C. R., Didas, S. A., & Jones, C. W.
Affiliations: Georgia Institute of Technology , , 311 Ferst Drive , , ,
Georgia Institute of Technology (US)
ORCID: Didas, Stephanie A.
Jones, Christopher W.
Venue: Chemical Reviews
Publisher: American Chemical Society (ACS)
Published: 2016-08-25
Volume: 116
Issue: 19
Pages: 11840-11876
ISSN: 0009-2665 (ISSN-L)
1520-6890
DOI: 10.1021/acs.chemrev.6b00173
OpenAlex: W2508859475
Semantic Scholar: 1730cf009126df0e913e24859aaee075b31b6a00
Cited by: 2,406
References: 238
Citations by year: 2026: 325 · 2025: 350 · 2024: 335 · 2023: 281 · 2022: 263 · 2021: 257 · 2020: 223 · 2019: 158 · 2018: 119 · 2017: 87 · 2016: 7
FWCI: 11.84
Type: journal article
Language: en
Open access: hybrid
doi.org
Licence: other-oa
pubs.acs.org/page/policy/authorchoice_termsofuse.html (vor)
Locations: Chemical Reviews (publishedVersion, other-oa)
PubMed (publishedVersion)
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Funders: Basic Energy Sciences (DE-SC0012577)
Topics: Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
Keywords: direct air capture, CO2 capture, basic solvents, metal-organic frameworks, sorption-desorption cycles, climate change mitigation, techno-economic analysis
MeSH terms: Adsorption, Air, Alkalies, Amines, Carbon Dioxide, Coordination Complexes

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Direct Capture of CO2 from Ambient Air

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