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Effects of Aqueous-Phase and Photochemical Processing on Secondary Organic Aerosol Formation and Evolution in Beijing, China
Abstract
Secondary organic aerosol (SOA) constitutes a large fraction of OA, yet remains a source of significant uncertainties in climate models due to incomplete understanding of its formation mechanisms and evolutionary processes. Here we evaluated the effects of photochemical and aqueous-phase processing on SOA composition and oxidation degrees in three seasons in Beijing, China, using high-resolution aerosol mass spectrometer measurements along with positive matrix factorization. Our results show that aqueous-phase processing has a dominant impact on the formation of more oxidized SOA (MO–OOA), and the contribution of MO–OOA to OA increases substantially as a function of relative humidity or liquid water content. In contrast, photochemical processing plays a major role in the formation of less oxidized SOA (LO–OOA), as indicated by the strong correlations between LO–OOA and odd oxygen (O x = O 3 + NO 2 ) during periods of photochemical production (R 2 = 0.59–0.80). Higher oxygen-to-carbon ratios of SOA during periods with higher RH were also found indicating a major role of aqueous-phase processing in changing the oxidation degree of SOA in Beijing. Episodes analyses further highlight that LO–OOA plays a more important role during the early stage of the formation of autumn/winter haze episodes while MO–OOA is more significant during the later evolution period.
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Cites
Paatero, P., & Tapper, U. (1994) · Environmetrics · doi:10.1002/env.3170050203 · Cited by 6,023
High secondary aerosol contribution to particulate pollution during haze events in China
Huang, R.-J., Zhang, Y., Bozzetti, C., Ho, K.-F., Cao, J.-J., Han, Y., Daellenbach, K. R., Slowik, J. G., Platt, S. M., Canonaco, F., et al. (2014) · Nature · doi:10.1038/nature13774 · Cited by 4,556
Self-citationEvolution of Organic Aerosols in the Atmosphere
Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., et al. (2009) · Science · doi:10.1126/science.1180353 · Cited by 4,167
Self-citationOrganic aerosol and global climate modelling: a review
Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., Van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., et al. (2005) · Atmospheric Chemistry and Physics · doi:10.5194/acp-5-1053-2005 · Cited by 3,244
Zhang, Q., Jimenez, J. L., Canagaratna, M. R., Allan, J. D., Coe, H., Ulbrich, I., Alfarra, M. R., Takami, A., Middlebrook, A. M., Sun, Y. L., et al. (2007) · Geophysical Research Letters · doi:10.1029/2007gl029979 · Cited by 2,452
Self-citationFountoukis, C., & Nenes, A. (2007) · Atmospheric Chemistry and Physics · doi:10.5194/acp-7-4639-2007 · Cited by 1,800
Elucidating severe urban haze formation in China
Guo, S., Hu, M., Zamora, M. L., Peng, J., Shang, D., Zheng, J., Du, Z., Wu, Z., Shao, M., Zeng, L., et al. (2014) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1419604111 · Cited by 1,711
Development of an Aerosol Mass Spectrometer for Size and Composition Analysis of Submicron Particles
Jayne, J. T., Leard, D. C., Zhang, X., Davidovits, P., Smith, K. A., Kolb, C. E., & Worsnop, D. R. (2000) · Aerosol Science and Technology · doi:10.1080/027868200410840 · Cited by 1,604
Self-citationCoupled Partitioning, Dilution, and Chemical Aging of Semivolatile Organics
Donahue, N. M., Robinson, A. L., Stanier, C. O., & Pandis, S. N. (2006) · Environmental Science & Technology · doi:10.1021/es052297c · Cited by 1,525
Aiken, A. C., DeCarlo, P. F., Kroll, J. H., Worsnop, D. R., Huffman, J. A., Docherty, K. S., Ulbrich, I. M., Mohr, C., Kimmel, J. R., Sueper, D., et al. (2008) · Environmental Science & Technology · doi:10.1021/es703009q · Cited by 1,492
Self-citationErvens, B., Turpin, B. J., & Weber, R. J. (2011) · Atmospheric Chemistry and Physics · doi:10.5194/acp-11-11069-2011 · Cited by 1,319
Canagaratna, M. R., Jimenez, J. L., Kroll, J. H., Chen, Q., Kessler, S. H., Massoli, P., Hildebrandt Ruiz, L., Fortner, E., Williams, L. R., Wilson, K. R., et al. (2015) · Atmospheric Chemistry and Physics · doi:10.5194/acp-15-253-2015 · Cited by 1,013
Self-citationAmbient aerosol sampling using the Aerodyne Aerosol Mass Spectrometer
Jimenez, J. L., Jayne, J. T., Shi, Q., Kolb, C. E., Worsnop, D. R., Yourshaw, I., Seinfeld, J. H., Flagan, R. C., Zhang, X., Smith, K. A., et al. (2003) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2001jd001213 · Cited by 942
Self-citationZhang, Q., Jimenez, J. L., Canagaratna, M. R., Ulbrich, I. M., Ng, N. L., Worsnop, D. R., & Sun, Y. (2011) · Analytical and Bioanalytical Chemistry · doi:10.1007/s00216-011-5355-y · Cited by 924
Self-citationDrewnick, F., Hings, S. S., DeCarlo, P., Jayne, J. T., Gonin, M., Fuhrer, K., Weimer, S., Jimenez, J. L., Demerjian, K. L., Borrmann, S., et al. (2005) · Aerosol Science and Technology · doi:10.1080/02786820500182040 · Cited by 730
Self-citationSun, Y., Jiang, Q., Wang, Z., Fu, P., Li, J., Yang, T., & Yin, Y. (2014) · Journal of Geophysical Research: Atmospheres · doi:10.1002/2014jd021641 · Cited by 715
Self-citationAqueous chemistry and its role in secondary organic aerosol (SOA) formation
Lim, Y. B., Tan, Y., Perri, M. J., Seitzinger, S. P., & Turpin, B. J. (2010) · Atmospheric Chemistry and Physics · doi:10.5194/acp-10-10521-2010 · Cited by 585
Aerosol composition, sources and processes during wintertime in Beijing, China
Sun, Y. L., Wang, Z. F., Fu, P. Q., Yang, T., Jiang, Q., Dong, H. B., Li, J., & Jia, J. J. (2013) · Atmospheric Chemistry and Physics · doi:10.5194/acp-13-4577-2013 · Cited by 574
Self-citationOrganic Atmospheric Particulate Material
Seinfeld, J. H., & Pankow, J. F. (2003) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.54.011002.103756 · Cited by 561
Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S., Reff, A., Lim, H.-J., & Ervens, B. (2007) · Atmospheric Environment · doi:10.1016/j.atmosenv.2007.05.035 · Cited by 550
Dimethyl Sulfide and Dimethyl Sulfoxide and Their Oxidation in the Atmosphere
Barnes, I., Hjorth, J., & Mihalopoulos, N. (2006) · Chemical Reviews · doi:10.1021/cr020529+ · Cited by 544
A simplified description of the evolution of organic aerosol composition in the atmosphere
Heald, C. L., Kroll, J. H., Jimenez, J. L., Docherty, K. S., DeCarlo, P. F., Aiken, A. C., Chen, Q., Martin, S. T., Farmer, D. K., & Artaxo, P. (2010) · Geophysical Research Letters · doi:10.1029/2010gl042737 · Cited by 511
Sun, Y.-L., Zhang, Q., Schwab, J. J., Demerjian, K. L., Chen, W.-N., Bae, M.-S., Hung, H.-M., Hogrefe, O., Frank, B., Rattigan, O. V., et al. (2011) · Atmospheric Chemistry and Physics · doi:10.5194/acp-11-1581-2011 · Cited by 452
Self-citationSun, Y., Wang, Z., Fu, P., Jiang, Q., Yang, T., Li, J., & Ge, X. (2013) · Atmospheric Environment · doi:10.1016/j.atmosenv.2013.06.019 · Cited by 406
Self-citationHu, W., Hu, M., Hu, W., Jimenez, J. L., Yuan, B., Chen, W., Wang, M., Wu, Y., Chen, C., Wang, Z., et al. (2016) · Journal of Geophysical Research: Atmospheres · doi:10.1002/2015jd024020 · Cited by 401
Self-citationPrimary and secondary aerosols in Beijing in winter: sources, variations and processes
Sun, Y., Du, W., Fu, P., Wang, Q., Li, J., Ge, X., Zhang, Q., Zhu, C., Ren, L., Xu, W., et al. (2016) · Atmospheric Chemistry and Physics · doi:10.5194/acp-16-8309-2016 · Cited by 393
Self-citationElser, M., Huang, R.-J., Wolf, R., Slowik, J. G., Wang, Q., Canonaco, F., Li, G., Bozzetti, C., Daellenbach, K. R., Huang, Y., et al. (2016) · Atmospheric Chemistry and Physics · doi:10.5194/acp-16-3207-2016 · Cited by 389
Self-citationMatthew, B. M., Middlebrook, A. M., & Onasch, T. B. (2008) · Aerosol Science and Technology · doi:10.1080/02786820802356797 · Cited by 357
A Case Study of Urban Particle Acidity and Its Influence on Secondary Organic Aerosol
Zhang, Q., Jimenez, J. L., Worsnop, D. R., & Canagaratna, M. (2007) · Environmental Science & Technology · doi:10.1021/es061812j · Cited by 352
Self-citationSources and properties of Amazonian aerosol particles
Martin, S. T., Andreae, M. O., Artaxo, P., Baumgardner, D., Chen, Q., Goldstein, A. H., Guenther, A., Heald, C. L., Mayol-Bracero, O. L., McMurry, P. H., et al. (2010) · Reviews of Geophysics · doi:10.1029/2008rg000280 · Cited by 347
Relating hygroscopicity and composition of organic aerosol particulate matter
Duplissy, J., DeCarlo, P. F., Dommen, J., Alfarra, M. R., Metzger, A., Barmpadimos, I., Prevot, A. S. H., Weingartner, E., Tritscher, T., Gysel, M., et al. (2011) · Atmospheric Chemistry and Physics · doi:10.5194/acp-11-1155-2011 · Cited by 340
Self-citationAltieri, K. E., Seitzinger, S. P., Carlton, A. G., Turpin, B. J., Klein, G. C., & Marshall, A. G. (2007) · Atmospheric Environment · doi:10.1016/j.atmosenv.2007.11.015 · Cited by 336
Characterization of submicron aerosols during a month of serious pollution in Beijing, 2013
Zhang, J. K., Sun, Y., Liu, Z. R., Ji, D. S., Hu, B., Liu, Q., & Wang, Y. S. (2014) · Atmospheric Chemistry and Physics · doi:10.5194/acp-14-2887-2014 · Cited by 319
Self-citationSun, Y., Wang, Z., Dong, H., Yang, T., Li, J., Pan, X., Chen, P., & Jayne, J. T. (2012) · Atmospheric Environment · doi:10.1016/j.atmosenv.2012.01.013 · Cited by 316
Self-citationOrganic aerosol composition and sources in Pasadena, California, during the 2010 CalNex campaign
Hayes, P. L., Ortega, A. M., Cubison, M. J., Froyd, K. D., Zhao, Y., Cliff, S. S., Hu, W. W., Toohey, D. W., Flynn, J. H., Lefer, B. L., et al. (2013) · Journal of Geophysical Research: Atmospheres · doi:10.1002/jgrd.50530 · Cited by 298
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Kondo, Y., Miyazaki, Y., Takegawa, N., Miyakawa, T., Weber, R. J., Jimenez, J. L., Zhang, Q., & Worsnop, D. R. (2007) · Journal of Geophysical Research: Atmospheres · doi:10.1029/2006jd007056 · Cited by 297
Self-citationRapid formation and evolution of an extreme haze episode in Northern China during winter 2015
Sun, Y., Chen, C., Zhang, Y., Xu, W., Zhou, L., Cheng, X., Zheng, H., Ji, D., Li, J., Tang, X., et al. (2016) · Scientific Reports · doi:10.1038/srep27151 · Cited by 273
Self-citationLoading-dependent elemental composition of α-pinene SOA particles
Shilling, J. E., Chen, Q., King, S. M., Rosenoern, T., Kroll, J. H., Worsnop, D. R., DeCarlo, P. F., Aiken, A. C., Sueper, D., Jimenez, J. L., et al. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-771-2009 · Cited by 249
Self-citationThe time evolution of aerosol composition over the Mexico City plateau
Kleinman, L. I., Springston, S. R., Daum, P. H., Lee, Y.-N., Nunnermacker, L. J., Senum, G. I., Wang, J., Weinstein-Lloyd, J., Alexander, M. L., Hubbe, J., et al. (2008) · Atmospheric Chemistry and Physics · doi:10.5194/acp-8-1559-2008 · Cited by 232
Ge, X., Zhang, Q., Sun, Y., Ruehl, C. R., & Setyan, A. (2012) · Environmental Chemistry · doi:10.1071/en11168 · Cited by 200
Self-citationCorrelation of secondary organic aerosol with odd oxygen in Mexico City
Herndon, S. C., Onasch, T. B., Wood, E. C., Kroll, J. H., Canagaratna, M. R., Jayne, J. T., Zavala, M. A., Knighton, W. B., Mazzoleni, C., Dubey, M. K., et al. (2008) · Geophysical Research Letters · doi:10.1029/2008gl034058 · Cited by 197
Self-citationEnhanced secondary organic aerosol formation due to water uptake by fine particles
Hennigan, C. J., Bergin, M. H., Dibb, J. E., & Weber, R. J. (2008) · Geophysical Research Letters · doi:10.1029/2008gl035046 · Cited by 193
Sorooshian, A., Murphy, S. M., Hersey, S., Bahreini, R., Jonsson, H., Flagan, R. C., & Seinfeld, J. H. (2010) · Geophysical Research Letters · doi:10.1029/2010gl044951 · Cited by 184
Secondary Organic Aerosol: A Comparison between Foggy and Nonfoggy Days
Kaul, D. S., Gupta, T., Tripathi, S. N., Tare, V., & Collett, J. L. (2011) · Environmental Science & Technology · doi:10.1021/es201081d · Cited by 171
Zorn, S. R., Drewnick, F., Schott, M., Hoffmann, T., & Borrmann, S. (2008) · Atmospheric chemistry and physics · doi:10.5194/acp-8-4711-2008 · Cited by 169
Gas/particle partitioning of water-soluble organic aerosol in Atlanta
Hennigan, C. J., Bergin, M. H., Russell, A. G., Nenes, A., & Weber, R. J. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-3613-2009 · Cited by 165
Chen, Q., Liu, Y., Donahue, N. M., Shilling, J. E., & Martin, S. T. (2011) · Environmental Science & Technology · doi:10.1021/es104398s · Cited by 161
Xu, W., Sun, Y., Chen, C., Du, W., Han, T. T., Wang, Q. Q., Fu, P., Wang, Z. F., Zhao, X., Zhou, L., et al. (2015) · Atmospheric chemistry and physics · doi:10.5194/acp-15-13681-2015 · Cited by 154
Self-citationWood, E. C., Canagaratna, M. R., Herndon, S. C., Onasch, T. B., Kolb, C. E., Worsnop, D. R., Kroll, J. H., Knighton, W. B., Seila, R. L., Zavala, M., et al. (2010) · Atmospheric chemistry and physics · doi:10.5194/acp-10-8947-2010 · Cited by 154
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Self-citationSun, Y.-L., Jiang, Q., Xu, Y., Ma, Y., Zhang, Y.-J., Liu, X.-G., Li, W.-J., Wang, F., Li, J., Wang, P.-C., et al. (2016) · Journal of Geophysical Research Atmospheres · doi:10.1002/2015jd024261 · Cited by 107
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Metadata
- Authors
- Xu, W., Han, T., Du, W., Wang, Q., Chen, C., Zhao, J., Zhang, Y., Li, J., Fu, P., Wang, Z., Worsnop, D. R., & Sun, Y.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-01-06
- Volume
- 51
- Issue
- 2
- Pages
- 762-770
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2567098959
- Cited by
- 317
- References
- 55
- FWCI
- 9.66
- Type
- journal article
- Language
- en
- Open access
- closed
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