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UiO-67-type Metal–Organic Frameworks with Enhanced Water Stability and Methane Adsorption Capacity
Abstract
The structure and properties of two new UiO-67-type metal-organic frameworks, along with their linker synthesis and powder and single crystal synthesis, are presented. The new MOFs, UiO-67-Me and UiO-67-BN, are based on 3,3'-dimethylbiphenyl and 1,1'-binaphthyl linker scaffolds, and show a much higher stability to water than the thoroughly investigated UiO-67, which is based on the biphenyl scaffold. On the basis of structure models obtained from single crystal X-ray diffraction, it is seen that these linkers are partly shielding the Zr cluster. The new materials have higher density than UiO-67, but show a higher volumetric adsorption capacity for methane. UiO-67-BN exhibits excellent reversible water sorption properties, and enhanced stability to aqueous solutions over a wide pH range; it is to the best of our knowledge the most stable Zr-MOF that is isostructural to UiO-67 in aqueous solutions.
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Cites
Crystal structure refinement with SHELXL
Sheldrick, G. M. (2015) · Acta Crystallographica Section C Structural Chemistry · doi:10.1107/s2053229614024218 · Cited by 43,982
Cited by
Shearer, G. C., Chavan, S., Bordiga, S., Svelle, S., Olsbye, U., & Lillerud, K. P. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b00602 · Cited by 1,437
Self-citationMetal–Organic Frameworks for Water Harvesting from Air
Kalmutzki, M. J., Diercks, C. S., & Yaghi, O. M. (2018) · Advanced Materials · doi:10.1002/adma.201704304 · Cited by 772
Ligand Rigidification for Enhancing the Stability of Metal–Organic Frameworks
Lv, X.-L., Yuan, S., Xie, L.-H., Darke, H. F., Chen, Y., He, T., Dong, C., Wang, B., Zhang, Y.-Z., Li, J.-R., et al. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b02947 · Cited by 322
Hydrophobic Metal–Organic Frameworks: Assessment, Construction, and Diverse Applications
Xie, L., Xu, M., Liu, X., Zhao, M., & Li, J. (2020) · Advanced Science · doi:10.1002/advs.201901758 · Cited by 284
Porous metal–organic frameworks for fuel storage
He, Y., Chen, F., Li, B., Qian, G., Zhou, W., & Chen, B. (2018) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.10.002 · Cited by 267
Metadata
- Authors
- Øien-Ødegaard, S., Bouchevreau, B., Hylland, K., Wu, L., Blom, R., Grande, C., Olsbye, U., Tilset, M., & Lillerud, K. P.
- Venue
- Inorganic Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-19
- Volume
- 55
- Issue
- 5
- Pages
- 1986-1991
- ISSN
- 0020-1669 (ISSN-L)
- 1520-510X
- OpenAlex
- W2278284344
- Cited by
- 159
- References
- 1
- FWCI
- 6.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Øien-Ødegaard, S., Bouchevreau, B., Hylland, K., Wu, L., Blom, R., Grande, C., Olsbye, U., Tilset, M., & Lillerud, K. P. (2016). UiO-67-type Metal–Organic Frameworks with Enhanced Water Stability and Methane Adsorption Capacity. Inorganic Chemistry. https://doi.org/10.1021/acs.inorgchem.5b02257
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