The DOI matches its Crossref record; 153 of the 153 references it cites were found in a registry or an index.
Application of Electrochemical Impedance Spectroscopy to Degradation and Aging Research of Lithium-Ion Batteries
Abstract
An in-depth understanding of battery degradation and aging in- Operando not only plays a vital role in the design of battery managing systems but also helps to ensure safe use and manufacturing optimization of lithium-ion batteries (LIBs) in large-scale applications. Electrochemical impedance spectroscopy (EIS) is a nondestructive method which unravels electrode kinetic processes inside the batteries in different time domains, including charge-transfer reactions, interfacial evolutions, and mass diffusions. It has become a powerful diagnosis and pre/prognosis tool in battery aging research, as it provides important insight into the changes of internal electrochemical processes by correlating the impedance evolution to degradation mechanisms. This review gives a critical overview on rapidly developing impedance techniques for degradation and aging investigation of Li-ion batteries. The EIS variations of LIBs at different aging conditions of calendar aging and accelerated aging are systematically summarized. In addition, the working principles, data validation, and modeling methods, including equivalent circuit model (ECM), distribution of relaxation times (DRT), and transmission line model (TLM), of classical EIS and dynamic EIS are elaborately concluded. Finally, the challenges and perspectives of further application of EIS in the aging research of LIBs are presented.
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Cites
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Electrochemical impedance spectroscopy
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Cited by
Aging mechanisms, prognostics and management for lithium-ion batteries: Recent advances
Wang, Y., Xiang, H., Soo, Y.-Y., & Fan, X. (2025) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2024.114915 · Cited by 142
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Physics-Based Battery Model Parametrisation from Impedance Data
Hallemans, N., Courtier, N. E., Please, C. P., Planden, B., Dhoot, R., Timms, R., Chapman, S. J., Howey, D., & Duncan, S. R. (2025) · Journal of The Electrochemical Society · doi:10.1149/1945-7111/add41b · Cited by 34
Metadata
- Authors
- Hu, W., Peng, Y., Wei, Y., & Yang, Y.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2023-03-01
- Volume
- 127
- Issue
- 9
- Pages
- 4465-4495
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W4322734451
- Cited by
- 429
- References
- 153
- FWCI
- 31.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, W., Peng, Y., Wei, Y., & Yang, Y. (2023). Application of Electrochemical Impedance Spectroscopy to Degradation and Aging Research of Lithium-Ion Batteries. The Journal of Physical Chemistry C. https://doi.org/10.1021/acs.jpcc.3c00033
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