Silicon Nanoantenna Mix Arrays for a Trifecta of Quantum Emitter Enhancements
Open accessAbstract
Dielectric nanostructures have demonstrated optical antenna effects due to Mie resonances. Previous work has exhibited enhancements in absorption, emission rates and directionality with practical limitations. In this paper, we present a Si mix antenna array to achieve a trifecta enhancement of ∼1200-fold with a Purcell factor of ∼47. The antenna design incorporates ∼10 nm gaps, within which fluorescent molecules strongly absorb the pump laser energy through a resonant mode. In the emission process, the antenna array increases the radiative decay rates of the fluorescence molecules via a Purcell effect and provides directional emission through a separate mode. This work could lead to novel CMOS-compatible platforms to enhance fluorescence for biological and chemical applications.
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
A novel nanophotonic platform based on dielectric nanostructures overcomes the limitations of plasmonic meta-surfaces.
“Via the realization of a novel nanophotonic platform based on dielectric nanostructures to form efficient nanoantennae with ultra-low light-into heat conversion, is demonstrated an approach that overcomes these limitations.”
From The Current State of Optical Sensors in Medical Wearables (2022) · cites this paper as [290]
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Cites
Resonance Absorption by Nuclear Magnetic Moments in a Solid
Purcell, E. M., Torrey, H. C., & Pound, R. V. (1946) · Physical Review · doi:10.1103/physrev.69.37 · Cited by 6,017 · see citing works
Optically resonant dielectric nanostructures
Kuznetsov, A. I., Miroshnichenko, A. E., Brongersma, M. L., Kivshar, Y. S., & Luk’yanchuk, B. (2016) · Science · doi:10.1126/science.aag2472 · Cited by 2,901 · see citing works
Self-citationDielectric Gradient Metasurface Optical Elements
Lin, D., Fan, P., Hasman, E., & Brongersma, M. L. (2014) · Science · doi:10.1126/science.1253213 · Cited by 2,371 · see citing works
Fluorescence quantum yields of some rhodamine dyes
Kubin, R. F., & Fletcher, A. N. (1982) · Journal of Luminescence · doi:10.1016/0022-2313(82)90045-x · Cited by 1,223 · see citing works
Directional visible light scattering by silicon nanoparticles
Fu, Y. H., Kuznetsov, A. I., Miroshnichenko, A. E., Yu, Y., & Luk’yanchuk, B. (2013) · Nature Communications · doi:10.1038/ncomms2538 · Cited by 1,128 · see citing works
Self-citationKuznetsov, A. I., Miroshnichenko, A. E., Fu, Y. H., Zhang, J., & Luk’yanchuk, B. (2012) · Scientific Reports · doi:10.1038/srep00492 · Cited by 1,123 · see citing works
Self-citationProbing the mechanisms of large Purcell enhancement in plasmonic nanoantennas
Akselrod, G. M., Argyropoulos, C., Hoang, T. B., et al. (2014) · Nature Photonics · doi:10.1038/nphoton.2014.228 · Cited by 1,092 · see citing works
Demonstration of Magnetic Dipole Resonances of Dielectric Nanospheres in the Visible Region
Evlyukhin, A. B., Novikov, S. M., Zywietz, U., Eriksen, R. L., Reinhardt, C., Bozhevolnyi, S. I., & Chichkov, B. N. (2012) · Nano Letters · doi:10.1021/nl301594s · Cited by 1,005 · see citing works
Lasing action in strongly coupled plasmonic nanocavity arrays
Zhou, W. M., Dridi, M., Suh, J. Y., Kim, C. H., Co, D. T., Wasielewski, M. R., Schatz, G. C., & Odom, T. W. (2013) · Nature Nanotechnology · doi:10.1038/nnano.2013.99 · Cited by 805 · see citing works
Directional lasing in resonant semiconductor nanoantenna arrays
Ha, S. T., Fu, Y. H., Emani, N. K., Pan, Z., Bakker, R. M., Paniagua-Domínguez, R., & Kuznetsov, A. I. (2018) · Nature Nanotechnology · doi:10.1038/s41565-018-0245-5 · Cited by 605 · see citing works
Self-citationAll-dielectric optical nanoantennas
Krasnok, A., Miroshnichenko, A. E., Belov, P. A., et al. (2012) · Optics Express · doi:10.1364/oe.20.020599 · Cited by 560 · see citing works
Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., Oulton, R. F., Bragas, A. V., & Maier, S. A. (2015) · Nature Communications · doi:10.1038/ncomms8915 · Cited by 520 · see citing works
Demonstration of Zero Optical Backscattering from Single Nanoparticles
Person, S., Jain, M., Lapin, Z. J., Sáenz, J. J., Wicks, G. W., & Novotný, L. (2013) · Nano Letters · doi:10.1021/nl4005018 · Cited by 507 · see citing works
Ultrafast All-Optical Switching with Magnetic Resonances in Nonlinear Dielectric Nanostructures
Shcherbakov, M. R., Vabishchevich, P. P., Shorokhov, A. S., et al. (2015) · Nano Letters · doi:10.1021/acs.nanolett.5b02989 · Cited by 442 · see citing works
Magnetic and Electric Hotspots with Silicon Nanodimers
Bakker, R. M., Permyakov, D. V., Yu, Y., Markovich, D., Paniagua-Domínguez, R. J., Gonzaga, L. V., Samusev, A. K., Kivshar, Y. S., Luk’yanchuk, B., & Kuznetsov, A. I. (2015) · Nano Letters · doi:10.1021/acs.nanolett.5b00128 · Cited by 419 · see citing works
Self-citationOn the Energy Shift between Near-Field and Far-Field Peak Intensities in Localized Plasmon Systems
Zuloaga, J., & Nordlander, P. J. (2011) · Nano Letters · doi:10.1021/nl1043242 · Cited by 370 · see citing works
Tuning the Color of Silicon Nanostructures
Cao, L., Fan, P., Barnard, E. S., Brown, A. M., & Brongersma, M. L. (2010) · Nano Letters · doi:10.1021/nl1013794 · Cited by 340 · see citing works
All-Dielectric Colored Metasurfaces with Silicon Mie Resonators
Proust, J., Bedu, F., Gallas, B., Ozerov, I., & Bonod, N. (2016) · ACS Nano · doi:10.1021/acsnano.6b03207 · Cited by 337 · see citing works
Printing Beyond sRGB Color Gamut by Mimicking Silicon Nanostructures in Free-Space
Dong, Z., Ho, J., Yu, Y. F., Fu, Y. H., Paniagua-Dominguez, R., Wang, S., Kuznetsov, A. I., & Yang, J. K. W. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b03613 · Cited by 335 · see citing works
Self-citationInteraction of Plasmon and Molecular Resonances for Rhodamine 6G Adsorbed on Silver Nanoparticles
Zhao, J., Jensen, L., Sung, J., Zou, S., Schatz, G. C., & Duyne, R. P. V. (2007) · Journal of the American Chemical Society · doi:10.1021/ja0707106 · Cited by 305 · see citing works
Trichromatic and Tripolarization-Channel Holography with Noninterleaved Dielectric Metasurface
Hu, Y., Li, L., Wang, Y., Meng, M., Jin, L., Luo, X., Chen, Y., Li, X., Xiao, S., Wang, H., et al. (2019) · Nano Letters · doi:10.1021/acs.nanolett.9b04107 · Cited by 290 · see citing works
Generalized Brewster effect in dielectric metasurfaces
Paniagua-Domínguez, R. J., Yu, Y., Miroshnichenko, A. E., Krivitsky, L. A., Fu, Y. H., Valuckas, V., Gonzaga, L. V., Toh, Y. T., Kay, A. Y. S., Luk’yanchuk, B., et al. (2016) · Nature Communications · doi:10.1038/ncomms10362 · Cited by 280 · see citing works
Self-citationAn all-dielectric metasurface as a broadband optical frequency mixer
Liu, S., Vabishchevich, P. P., Vaskin, A., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-04944-9 · Cited by 277 · see citing works
Koenderink, A. F. (2017) · ACS Photonics · doi:10.1021/acsphotonics.7b00061 · Cited by 276 · see citing works
Noninterleaved Metasurface for (26-1) Spin- and Wavelength-Encoded Holograms
Jin, L., Dong, Z., Mei, S., Yu, Y., Wei, Z., Pan, Z., Rezaei, S. D., Li, X., Kuznetsov, A. I., Kivshar, Y. S., et al. (2018) · Nano Letters · doi:10.1021/acs.nanolett.8b04246 · Cited by 258 · see citing works
Self-citationAnthur, A. P., Zhang, H., Paniagua-Domínguez, R. J., et al. (2020) · Nano Letters · doi:10.1021/acs.nanolett.0c03601 · Cited by 244 · see citing works
All-Dielectric Silicon Nanogap Antennas To Enhance the Fluorescence of Single Molecules
Regmi, R., Berthelot, J., Winkler, P. M., Mivelle, M., Proust, J., Bedu, F., Ozerov, I., Begou, T. C., Lumeau, J. H., Rigneault, H., et al. (2016) · Nano Letters · doi:10.1021/acs.nanolett.6b02076 · Cited by 238 · see citing works
Silicon multi‐meta‐holograms for the broadband visible light
Huang, K., Dong, Z., Mei, S., Zhang, L., Liu, Y., Liu, H., Zhu, H., Teng, J., Luk’yanchuk, B., Yang, J. K. W., et al. (2016) · Laser & Photonics Review · doi:10.1002/lpor.201500314 · Cited by 230 · see citing works
Self-citationSilicon Mie resonators for highly directional light emission from monolayer MoS2
Cihan, A. F., Curto, A. G., Raza, S., et al. (2018) · Nature Photonics · doi:10.1038/s41566-018-0155-y · Cited by 212 · see citing works
Metallic nanostructures for efficient LED lighting
Lozano, G., Rodriguez, S., Verschuuren, M. A., et al. (2016) · Light Science & Applications · doi:10.1038/lsa.2016.80 · Cited by 199 · see citing works
Silicon Nanostructures for Bright Field Full Color Prints
Flauraud, V., Reyes, M., Paniagua-Domínguez, R. J., Kuznetsov, A. I., & Brügger, J. (2017) · ACS Photonics · doi:10.1021/acsphotonics.6b01021 · Cited by 198 · see citing works
Self-citationAll-Dielectric Dual-Color Pixel with Subwavelength Resolution
Nagasaki, Y., Suzuki, M., & Takahara, J. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b03421 · Cited by 194 · see citing works
Efficient Second-Harmonic Generation in Nanocrystalline Silicon Nanoparticles
Makarov, S., Petrov, M. I., Zywietz, U., Milichko, V. A., Zuev, D. A., Lopanitsyna, N., Kuksin, A. Y., Mukhin, I. S., Zograf, G., Убыйвовк, Е. В., et al. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b00392 · Cited by 193 · see citing works
Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation
Liu, S., Vaskin, A., Addamane, S., et al. (2018) · Nano Letters · doi:10.1021/acs.nanolett.8b02808 · Cited by 191 · see citing works
Meng, J., Cadusch, J. J., & Crozier, K. B. (2019) · Nano Letters · doi:10.1021/acs.nanolett.9b03862 · Cited by 176 · see citing works
Quantum Dot Emission Driven by Mie Resonances in Silicon Nanostructures
Rutckaia, V., Heyroth, F., Novikov, A. V., Shaleev, M. V., Petrov, M. I., & Schilling, J. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b03248 · Cited by 163 · see citing works
Chen, Y., Bi, K., Wang, Q., et al. (2016) · ACS Nano · doi:10.1021/acsnano.6b06290 · Cited by 161 · see citing works
Strong Photoluminescence Enhancement in All-Dielectric Fano Metasurface with High Quality Factor
Yuan, S., Qiu, X.-Z., Cui, C., Zhu, L., Wang, Y., Li, Y., Song, J., Huang, Q., & Xia, J. (2017) · ACS Nano · doi:10.1021/acsnano.7b04810 · Cited by 150 · see citing works
Active Tuning of Spontaneous Emission by Mie-Resonant Dielectric Metasurfaces
Bohn, J., Bucher, T., Chong, K. E., Komar, A., Choi, D., Neshev, D. N., Kivshar, Y. S., Pertsch, T., & Staude, I. (2018) · Nano Letters · doi:10.1021/acs.nanolett.8b00475 · Cited by 144 · see citing works
Shaping Photoluminescence Spectra with Magnetoelectric Resonances in All-Dielectric Nanoparticles
Staude, I., Khardikov, V. V., Fofang, N. T., et al. (2015) · ACS Photonics · doi:10.1021/ph500379p · Cited by 137 · see citing works
Yang, Y., Yoon, G., Park, S., Namgung, S. D., Badloe, T., Nam, K. T., & Rho, J. (2021) · Advanced Materials · doi:10.1002/adma.202005893 · Cited by 113 · see citing works
Tailoring Photoluminescence from MoS2 Monolayers by Mie-Resonant Metasurfaces
Bucher, T., Vaskin, A., Mupparapu, R., et al. (2019) · ACS Photonics · doi:10.1021/acsphotonics.8b01771 · Cited by 112 · see citing works
Electrically-driven Yagi-Uda antennas for light
Kullock, R., Ochs, M., Grimm, P., et al. (2020) · Nature Communications · doi:10.1038/s41467-019-14011-6 · Cited by 112 · see citing works
Tailor-made directional emission in nanoimprinted plasmonic-based light-emitting devices
Lozano, G., Grzela, G., Verschuuren, M. A., et al. (2014) · Nanoscale · doi:10.1039/c4nr01391c · Cited by 111 · see citing works
All-Dielectric Metasurface Fluorescence Biosensors for High-Sensitivity Antibody/Antigen Detection
Iwanaga, M. (2020) · ACS Nano · doi:10.1021/acsnano.0c07722 · Cited by 108 · see citing works
Dong, Z., Asbahi, M., Lin, J., Zhu, D., Wang, Y. M., Hippalgaonkar, K., Chu, H., Goh, W. P., Wang, F., Huang, Z., et al. (2015) · Nano Letters · doi:10.1021/acs.nanolett.5b02109 · Cited by 102 · see citing works
Self-citationBelushkin, A. A., Yesilköy, F., González‐López, J. J., Ruiz‐Rodríguez, J. C., Ferrer, R., Fàbrega, A., & Altug, H. (2019) · Small · doi:10.1002/smll.201906108 · Cited by 98 · see citing works
Unidirectional Doubly Enhanced MoS2 Emission via Photonic Fano Resonances
Zhang, X., Choi, S., Wang, D., et al. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b02777 · Cited by 95 · see citing works
Enhanced Light Emission by Magnetic and Electric Resonances in Dielectric Metasurfaces
Murai, S., Castellanos, G. W., Raziman, T. V., et al. (2020) · Advanced Optical Materials · doi:10.1002/adom.201902024 · Cited by 93 · see citing works
Fabri-Faja, N., Calvo-Lozano, O., Dey, P., et al. (2019) · Analytica Chimica Acta · doi:10.1016/j.aca.2019.05.038 · Cited by 92 · see citing works
Broadband Dielectric–Metal Hybrid Nanoantenna: Silicon Nanoparticle on a Mirror
Sugimoto, H., & Fujii, M. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b01461 · Cited by 89 · see citing works
“Sketch and Peel” Lithography for High-Resolution Multiscale Patterning
Chen, Y., Xiang, Q., Li, Z., et al. (2016) · Nano Letters · doi:10.1021/acs.nanolett.6b00788 · Cited by 77 · see citing works
Ultraviolet Interband Plasmonics With Si Nanostructures
Dong, Z., Wang, T., Chi, X., Ho, J., Tserkezis, C., Yap, S. L. K., Rusydi, A., Tjiptoharsono, F., Thian, D., Mortensen, N. A., et al. (2019) · Nano Letters · doi:10.1021/acs.nanolett.9b03243 · Cited by 71 · see citing works
Self-citationStructural Evolution of Ultrathin Films of Rhodamine 6G on Glass
Chapman, M., Mullen, M., Novoa-Ortega, E., Alhasani, M. A., Elman, J. F., & Euler, W. B. (2016) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.6b01669 · Cited by 53 · see citing works
Chen, H., Nanz, S., Abass, A., Yan, J., Gao, T., Choi, D., Kivshar, Y. S., Rockstuhl, C., & Neshev, D. N. (2017) · ACS Photonics · doi:10.1021/acsphotonics.7b00550 · Cited by 50 · see citing works
Experimental Demonstration of In-Plane Negative-Angle Refraction with an Array of Silicon Nanoposts
Wu, A., Li, H., Du, J., et al. (2015) · Nano Letters · doi:10.1021/nl5049516 · Cited by 44 · see citing works
Raman analysis of three-dimensionally graded stress tensor components in sapphire
Zhu, W., & Pezzotti, G. (2011) · Journal of Applied Physics · doi:10.1063/1.3559871 · Cited by 38 · see citing works
Electrically-Excited Surface Plasmon Polaritons with Directionality Control
Dong, Z., Chu, H., Zhu, D., Du, W., Akimov, Y., Goh, W. P., Wang, T., Goh, K. E. J., Troadec, C., Nijhuis, C. A., et al. (2015) · ACS Photonics · doi:10.1021/ph5004303 · Cited by 38 · see citing works
Self-citationUnidirectional Enhanced Emission from 2D Monolayer Suspended by Dielectric Pillar Array
Ao, X., Xu, X., Dong, J., & He, S. (2018) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.8b12701 · Cited by 20 · see citing works
Large area metasurfaces made with spherical silicon resonators
Molet, P., Gil-Herrera, L. K., García‐Pomar, J. L., et al. (2020) · Nanophotonics · doi:10.1515/nanoph-2020-0035 · Cited by 18 · see citing works
Highly Directional Fluorescent Emission at Visible Wavelengths with a Silicon Metasurface
Song, W., Li, S., & Crozier, K. B. (2016) · Conference on Lasers and Electro-Optics · doi:10.1364/cleo_qels.2016.fm3d.7 · Cited by 2 · see citing works
Flagged first, then by citations
Research works printed but not linked: 1
- Chapman, M.; Mullen, M., et al. Structural Evolution of Ultrathin Films of Rhodamine 6G on Glass, The Journal of Physical Chemistry C 2016, 120, (15), 8289-8297.
Cited by
Sorted by citations
The Current State of Optical Sensors in Medical Wearables
Vavrinsky, E., Esfahani, N. E., Hausner, M., Kuzma, A., Rezo, V., Donoval, M., & Kosnacova, H. (2022) · Biosensors · doi:10.3390/bios12040217 · Cited by 103 · see citing works
- Authors
- Dong, Z., Gorelik, S., Paniagua-Dominguez, R., Yik, J., Ho, J., Tjiptoharsono, F., Lassalle, E., Rezaei, S. D., Neo, D. C. J., Bai, P., Kuznetsov, A. I., & Yang, J. K. W.
- Affiliations
- Agency for Science, Technology and Research (SG)
- Institute of Materials Research and Engineering, A*STAR (Agency for Science, Technology and Research), 2 Fusionopolis Way, #08-03 Innovis, 138634 Singapore
- Singapore University of Technology and Design (SG)
- Corresponding author
- Dong, Zhaogang
- Kuznetsov, Arseniy I.
- Yang, Joel K. W.
- ORCID
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-05-27
- Volume
- 21
- Issue
- 11
- Pages
- 4853-4860
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W3164062364
- Cited by
- 47
- References
- 61
- Citations by year
- 2026: 1 · 2025: 14 · 2024: 12 · 2023: 6 · 2022: 10 · 2021: 4
- FWCI
- 2.43
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Licence
- Locations
- Nano Letters (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- arXiv (Cornell University)
- Funders
- Agency for Science, Technology and Research (A*STAR career development award (CDA), A20E5c0093)
- Science and Engineering Research Council (1527300025)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Plasmonic and Surface Plasmon Research
- Physical Sciences › Engineering › Biomedical Engineering › Near-Field Optical Microscopy
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Photonic and Optical Devices
- Keywords
- silicon nanoantennas, antenna arrays, Purcell effect, Mie resonance, dielectric nanostructures, fluorescence enhancement, radiative decay rate, directional emission, nanogap, quantum emitters, CMOS-compatible photonics
- MeSH terms
- Fluorescence, Lasers, Light, Silicon, Nanostructures
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
