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Multilayer Graphene Enables Higher Efficiency in Improving Thermal Conductivities of Graphene/Epoxy Composites

Open access
Shen, Xi, Wang, Zhenyu, Wu, Ying, Liu, Xu, He, Yan-Bing, Kim, Jang-Kyo·2016·Nano Letters

Abstract

The effects of number of graphene layers (n) and size of multilayer graphene sheets on thermal conductivities (TCs) of their epoxy composites are investigated. Molecular dynamics simulations show that the in-plane TCs of graphene sheets and the TCs across the graphene/epoxy interface simultaneously increase with increasing n. However, such higher TCs of multilayer graphene sheets will not translate into higher TCs of bulk composites unless they have large lateral sizes to maintain their aspect ratios comparable to the monolayer counterparts. The benefits of using large, multilayer graphene sheets are confirmed by experiments, showing that the composites made from graphite nanoplatelets (n > 10) with over 30 μm in diameter deliver a TC of ∼1.5 W m(-1) K(-1) at only 2.8 vol %, consistently higher than those containing monolayer or few-layer graphene at the same graphene loading. Our findings offer a guideline to use cost-effective multilayer graphene as conductive fillers for various thermal management applications.

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Metadata

Authors
Shen, X., Wang, Z., Wu, Y., Liu, X., He, Y.-B., & Kim, J.-K.
Venue
Nano Letters
Published
2016-05-06
Volume
16
Issue
6
Pages
3585-3593
ISSN
  • 1530-6984 (ISSN-L)
  • 1530-6992
OpenAlex
W2346469363
Cited by
382
References
50
FWCI
19.79
Type
journal article
Language
en
Open access
hybrid

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CoChat. (2026). Citation check: Multilayer Graphene Enables Higher Efficiency in Improving Thermal Conductivities of Graphene/Epoxy Composites. https://app.cochat.ai/papers/10.1021/acs.nanolett.6b00722
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Shen, X., Wang, Z., Wu, Y., Liu, X., He, Y.-B., & Kim, J.-K. (2016). Multilayer Graphene Enables Higher Efficiency in Improving Thermal Conductivities of Graphene/Epoxy Composites. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b00722

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