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Morphological Engineering of Winged Au@MoS2 Heterostructures for Electrocatalytic Hydrogen Evolution
Open accessAbstract
Molybdenum disulfide (MoS 2 ) has been recognized as a promising cost-effective catalyst for water-splitting hydrogen production. However, the desired performance of MoS 2 is often limited by insufficient edge-terminated active sites, poor electrical conductivity, and inefficient contact to the supporting substrate. To address these limitations, we developed a unique nanoarchitecture (namely, winged Au@MoS 2 heterostructures enabled by our discovery of the “seeding effect” of Au nanoparticles for the chemical vapor deposition synthesis of vertically aligned few-layer MoS 2 wings). The winged Au@MoS 2 heterostructures provide an abundance of edge-terminated active sites and are found to exhibit dramatically improved electrocatalytic activity for the hydrogen evolution reaction. Theoretical simulations conducted for this unique heterostructure reveal that the hydrogen evolution is dominated by the proton adsorption step, which can be significantly promoted by introducing sufficient edge active sites. Our study introduces a new morphological engineering strategy to make the pristine MoS 2 layered structures highly competitive earth-abundant catalysts for efficient hydrogen production.
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Co9S8 is an attractive material for HER because of its good catalytic activity and stability.
“Co9S8 is regarded as an attractive material for HER because of its good catalytic activity and stability [24–33].”
From Synthesis of Au/Co9S8 composite aerogels by one-step sol–gel method as hydrogen evolution reaction electrocatalysts (2021) · cites this paper as [24]
The Abstract discusses MoS₂ as a promising HER material, and the structural-evolution section describes the activity and stability of winged Au@MoS₂ electrodes; neither addresses Co₉S₈. Searches for Co₉S₈ and cobalt sulfide found no passage assessing its HER activity or stability. Page numbers were not supplied for these passages. (LLM, conf=0.76)
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Metadata
- Authors
- Li, Y., Majewski, M. B., Islam, S. M., Hao, S., Murthy, A. A., DiStefano, J. G., Hanson, E. D., Xu, Y., Wolverton, C., Kanatzidis, M. G., Wasielewski, M. R., Chen, X., & Dravid, V. P.
- Affiliations
- Northwestern University (US)
- Corresponding author
- Chen, Xinqi
- Dravid, Vinayak P.
- ORCID
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-10-08
- Volume
- 18
- Issue
- 11
- Pages
- 7104-7110
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2896127892
- Cited by
- 115
- References
- 45
- Citations by year
- 2026: 4 · 2025: 10 · 2024: 7 · 2023: 14 · 2022: 18 · 2021: 15 · 2020: 22 · 2019: 24 · 2018: 1
- FWCI
- 3.58
- Type
- journal article
- Language
- en
- Open access
- green
- www.osti.gov
- Locations
- Nano Letters (publishedVersion)
- PubMed (publishedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- Northwestern University
- National Science Foundation
- Division of Materials Research (DMR-1507810)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Keywords
- MoS2, electrocatalytic hydrogen evolution, morphology engineering, chemical vapor deposition synthesis, proton adsorption, water splitting, earth-abundant catalysts
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