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Characterization of MoS2–Graphene Composites for High-Performance Coin Cell Supercapacitors
Open accessAbstract
Two-dimensional materials, such as graphene and molybdenum disulfide (MoS2), can greatly increase the performance of electrochemical energy storage devices because of the combination of high surface area and electrical conductivity. Here, we have investigated the performance of solution exfoliated MoS2 thin flexible membranes as supercapacitor electrodes in a symmetrical coin cell arrangement using an aqueous electrolyte (Na2SO4). By adding highly conductive graphene to form nanocomposite membranes, it was possible to increase the specific capacitance by reducing the resistivity of the electrode and altering the morphology of the membrane. With continued charge/discharge cycles the performance of the membranes was found to increase significantly (up to 800%), because of partial re-exfoliation of the layered material with continued ion intercalation, as well as increasing the specific capacitance through intercalation pseudocapacitance. These results demonstrate a simple and scalable application of layered 2D materials toward electrochemical energy storage.
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Two-dimensional atomic crystals
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Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts
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High yield exfoliation of two-dimensional chalcogenides using sodium naphthalenide
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Direct Laser‐Patterned Micro‐Supercapacitors from Paintable MoS2 Films
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Cited by
Samadi, M., Sarikhani, N., Zirak, M., Zhang, H., Zhang, H.-L., & Moshfegh, A. Z. (2018) · Nanoscale Horizons · doi:10.1039/c7nh00137a · Cited by 408
Dong, W., Xie, M., Zhao, S., Qin, Q., & Huang, F. (2023) · Materials Science and Engineering: R: Reports · doi:10.1016/j.mser.2022.100713 · Cited by 319
Highly Active 2D Layered MoS 2 -rGO Hybrids for Energy Conversion and Storage Applications
Kamila, S., Mohanty, B., Samantara, A. K., Guha, P., Ghosh, A., Jena, B., Satyam, P. V., Mishra, B. K., & Jena, B. K. (2017) · Scientific Reports · doi:10.1038/s41598-017-08677-5 · Cited by 189
Gigot, A., Fontana, M., Serrapede, M., Castellino, M., Bianco, S., Armandi, M., Bonelli, B., Pirri, C. F., Tresso, E., & Rivolo, P. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b11290 · Cited by 164
MoS 2 /MoO x ‐Nanostructure‐Decorated Activated Carbon Cloth for Enhanced Supercapacitor Performance
Sari, F. N. I., & Ting, J. (2018) · ChemSusChem · doi:10.1002/cssc.201702295 · Cited by 95
Metadata
- Authors
- Bissett, M. A., Kinloch, I. A., & Dryfe, R. A. W.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-07-31
- Volume
- 7
- Issue
- 31
- Pages
- 17388-17398
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2303258242
- Cited by
- 461
- References
- 6
- FWCI
- 16.27
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Bissett, M. A., Kinloch, I. A., & Dryfe, R. A. W. (2015). Characterization of MoS2–Graphene Composites for High-Performance Coin Cell Supercapacitors. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b04672
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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