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Fabrication and Enhanced Photoelectrochemical Performance of MoS2/S-Doped g-C3N4 Heterojunction Film

Ye, Lijuan, Wang, Dan, Chen, Shijian·2016·ACS Applied Materials & Interfaces

Abstract

We report on a novel MoS2/S-doped g-C3N4 heterojunction film with high visible-light photoelectrochemical (PEC) performance. The heterojunction films are prepared by CVD growth of S-doped g-C3N4 film on indium-tin oxide (ITO) glass substrates, with subsequent deposition of a low bandgap, 1.69 eV, visible-light response MoS2 layer by hydrothermal synthesis. Adding thiourea into melamine as the coprecursor not only facilitates the growth of g-C3N4 films but also introduces S dopants into the films, which significantly improves the PEC performance. The fabricated MoS2/S-doped g-C3N4 heterojunction film offers an enhanced anodic photocurrent of as high as ∼1.2 × 10(-4) A/cm(2) at an applied potential of +0.5 V vs Ag/AgCl under the visible light irradiation. The enhanced PEC performance of MoS2/S-doped g-C3N4 film is believed due to the improved light absorption and the efficient charge separation of the photogenerated charge at the MoS2/S-doped g-C3N4 interface. The convenient preparation of carbon nitride based heterojunction films in this work can be widely used to design new heterojunction photoelectrodes or photocatalysts with high performance for H2 evolution.

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Metadata

Authors
Ye, L., Wang, D., & Chen, S.
Venue
ACS Applied Materials & Interfaces
Published
2016-02-18
Volume
8
Issue
8
Pages
5280-5289
ISSN
  • 1944-8244 (ISSN-L)
  • 1944-8252
OpenAlex
W2274762352
Cited by
313
References
52
FWCI
11.80
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Fabrication and Enhanced Photoelectrochemical Performance of MoS2/S-Doped g-C3N4 Heterojunction Film. https://app.cochat.ai/papers/10.1021/acsami.5b11326
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Ye, L., Wang, D., & Chen, S. (2016). Fabrication and Enhanced Photoelectrochemical Performance of MoS2/S-Doped g-C3N4 Heterojunction Film. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b11326

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