Nanoparticle-Stacked Porous Nickel–Iron Nitride Nanosheet: A Highly Efficient Bifunctional Electrocatalyst for Overall Water Splitting
Abstract
Nanoparticle-stacked porous Ni3FeN nanosheets were synthesized through a simple nitridation reaction of the corresponding LDHs. The nanosheet is composed of stacked nanoparticles with more active sites exposed for electrocatalytic reactions. Thus, it exhibited excellent oxygen evolution reaction performance having an extremely low overpotential of 223 mV at 10 mA/cm(2) and hydrogen evolution reaction property with a very low overpotential of 45 mV at 10 mA/cm(2). This electrocatalyst as bifunctional electrodes is used to overall water splitting in alkaline media, showing a high performance with 10 mA/cm(2) at a cell voltage of 1.495 V.
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Ni3FeN (111) surfaces were used to construct a complex surface with r-GO because of the minimal surface energy of the (111) surface.
“The Ni3FeN (111) surfaces were used to construct a complex surface with r-GO because of the minimal surface energy of the (111) surface.22,23,43,44”
From Electronic Structure Tuning in Ni<sub>3</sub>FeN/r-GO Aerogel toward Bifunctional Electrocatalyst for Overall Water Splitting (2018) · cites this paper as [43]
Cites
Tian, N., Zhou, Z.-Y., Sun, S.-G., Ding, Y., & Wang, Z. L. (2007) · Science · doi:10.1126/science.1140484 · Cited by 3,073 · see citing works
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Gu, Y., Chen, S., Ren, J., Jia, Y. A., Chen, C., Komarneni, S., Yang, D., & Yao, X. (2018) · ACS Nano · doi:10.1021/acsnano.7b05971 · Cited by 540 · see citing works
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Ray, C., Lee, S. C., Sankar, K. V., Jin, B., Lee, J., Park, J. H., & Jun, S. C. (2017) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.7b11192 · Cited by 142 · see citing works
- Authors
- Wang, Y., Xie, C., Liu, D., Huang, X., Huo, J., & Wang, S.
- Affiliations
- Hunan University (CN)
- Hunan University of Arts and Science (CN)
- Corresponding author
- Wang, Shuangyin
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-07-12
- Volume
- 8
- Issue
- 29
- Pages
- 18652-18657
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2466191262
- Cited by
- 315
- References
- 2
- Citations by year
- 2026: 7 · 2025: 18 · 2024: 15 · 2023: 29 · 2022: 34 · 2021: 32 · 2020: 41 · 2019: 33 · 2018: 46 · 2017: 54 · 2016: 6
- FWCI
- 12.56
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Applied Materials & Interfaces (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Natural Science Foundation of China (21573066, 51402100)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Keywords
- porous nanosheets, layered double hydroxides, nitridation, bifunctional electrocatalysts, oxygen evolution reaction, hydrogen evolution reaction, overall water splitting, alkaline water electrolysis
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