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Cited by 215

The DOI matches its Crossref record; 20 of the 20 references it cites were found in a registry or an index.

Growth of One-Dimensional RuO2 Nanowires on g-Carbon Nitride: An Active and Stable Bifunctional Electrocatalyst for Hydrogen and Oxygen Evolution Reactions at All pH Values

Bhowmik, Tanmay, Kundu, Manas Kumar, Barman, Sudip·2016·ACS Applied Materials & Interfaces
DOI 10.1021/acsami.6b10436
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Abstract

Development of highly efficient and durable bifunctional electrocatalyst for hydrogen and oxygen evolution reactions (HER and OER) is essential for efficient solar fuel generation. The commercial RuO 2 or RuO 2 -based catalysts are highly active toward OER, but their poor stability under different operating conditions is the main obstacle for their commercialization. Herein, we report growth of one-dimensional highly crystalline RuO 2 nanowires on carbon nitride (1D-RuO 2 -CN x ) for their applications in HER and OER at all pH values. The 1D-RuO 2 -CN x, as an OER catalyst, exhibits a low onset overpotential of ∼200 mV in both acidic and basic media, whereas Tafel slopes are 52 and 56 mV/dec in acidic and basic media, respectively. This catalyst requires a low overpotential of 250 and 260 mV to drive the current density of 10 mA cm –2 in acidic and basic media, respectively. The mass activity of 1D-RuO 2 -CN x catalyst is 352 mA mg –1, which is ∼14 times higher than that of commercial RuO 2 . Most importantly, the 1D-RuO 2 -CN x catalyst has remarkably higher stability compared to commercial RuO 2 . This catalyst also exhibits superior HER activity with a current density of 10 mAcm –2 at ∼93 and 95 mV in acidic and basic media. The HER Tafel slopes of this catalyst are 40 mV/dec in acidic condition and 70 mV/dec in basic condition. The HER activity of this catalyst is slightly lower than Pt/C in acidic media, whereas in basic media it is comparable or even better than that of Pt/C at higher overpotentials. The HER stability of this catalyst is also better than that of Pt/C in all pH solutions. This superior catalytic activity of 1D-RuO 2 -CN x composite can be attributed to catalyst–support interaction, enhanced mass and electron transport, one-dimensional morphology, and highly crystalline rutile RuO 2 structure.

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Metadata

Authors
Bhowmik, T., Kundu, M. K., & Barman, S.
Venue
ACS Applied Materials & Interfaces
Publisher
American Chemical Society (ACS)
Published
2016-10-17
Volume
8
Issue
42
Pages
28678-28688
ISSN
  • 1944-8244 (ISSN-L)
  • 1944-8252
DOI
10.1021/acsami.6b10436
OpenAlex
W2528737532
Cited by
215
References
20
FWCI
4.92
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Growth of One-Dimensional RuO2 Nanowires on g-Carbon Nitride: An Active and Stable Bifunctional Electrocatalyst for Hydrogen and Oxygen Evolution Reactions at All pH Values. https://app.cochat.ai/papers/10.1021/acsami.6b10436
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Bhowmik, T., Kundu, M. K., & Barman, S. (2016). Growth of One-Dimensional RuO2 Nanowires on g-Carbon Nitride: An Active and Stable Bifunctional Electrocatalyst for Hydrogen and Oxygen Evolution Reactions at All pH Values. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.6b10436

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