The DOI matches its Crossref record; 54 of the 54 references it cites were found in a registry or an index.
Mixed 1T–2H Phase MoS2/Reduced Graphene Oxide as Active Electrode for Enhanced Supercapacitive Performance
Abstract
A hybrid aerogel, composed of MoS 2 sheets of 1T (distorted octahedral) and 2H (trigonal prismatic) phases, finely mixed with few layers of reduced graphene oxide (rGO) and obtained by means of a facile environment-friendly hydrothermal cosynthesis, is proposed as electrode material for supercapacitors. By electrochemical characterizations in three- and two-electrode configurations and symmetric planar devices, unique results have been obtained, with specific capacitance values up to 416 F g -1 and a highly stable capacitance behavior over 50000 charge-discharge cycles. The in-depth morphological and structural characterizations through field emission scanning electron microscopy, Raman, X-ray photoelectron spectroscopy, X-ray diffraction, Brunauer-Emmett-Teller, and transmission electron microscopy analysis provides the proofs of the unique assembly of such 3D structured matrix. The unpacked MoS 2 structure exhibits an excellent distribution of 1T and 2H phase sheets that are highly exposed to interaction with the electrolyte, and so available for surface/near-surface redox reactions, notwithstanding the quite low overall content of MoS 2 embedded in the reduced graphene oxide (rGO) matrix. A comparison with other "more conventional" hybrid rGO-MoX 2 electrochemically active materials, synthesized in the same conditions, is provided to support the outstanding behavior of the cosynthesized rGO-MoS 2 .
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“Such graphene-based nanocomposites have the potential to ameliorate energy storage devices by leveraging the ample specific surface area of graphene and Faradaic redox reactions of TMDs or LDHs.27−32”
From Integrated Energy Aerogel of N,S-rGO/WSe 2 /NiFe-LDH for Both Energy Conversion and Storage (2017) · cites this paper as [27]
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Transition Metal Sulfides Based on Graphene for Electrochemical Energy Storage
Geng, P., Zheng, S., Tang, H., Zhu, R., Zhang, L., Cao, S., Xue, H., & Pang, H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201703259 · Cited by 864
Pham, P. V., Bodepudi, S. C., Shehzad, K., Liu, Y., Xu, Y., Yu, B., & Duan, X. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00735 · Cited by 736
Recent Development of Metallic (1T) Phase of Molybdenum Disulfide for Energy Conversion and Storage
Lei, Z., Zhan, J., Tang, L., Zhang, Y., & Wang, Y. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201703482 · Cited by 488
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Design Strategies for Development of TMD-Based Heterostructures in Electrochemical Energy Systems
Prabhu, P., Jose, V., & Lee, J.-M. (2020) · Matter · doi:10.1016/j.matt.2020.01.001 · Cited by 460
Metadata
- Authors
- Gigot, A., Fontana, M., Serrapede, M., Castellino, M., Bianco, S., Armandi, M., Bonelli, B., Pirri, C. F., Tresso, E., & Rivolo, P.
- Affiliations
- Politecnico di Torino (IT)
- Italian Institute of Technology (IT)
- Corresponding author
- Rivolo, Paola
- ORCID
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-11-21
- Volume
- 8
- Issue
- 48
- Pages
- 32842-32852
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2553462613
- Cited by
- 164
- References
- 54
- Citations by year
- 2026: 9 · 2025: 14 · 2024: 14 · 2023: 17 · 2022: 19 · 2021: 10 · 2020: 25 · 2019: 19 · 2018: 30 · 2017: 7
- FWCI
- 5.87
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Applied Materials & Interfaces (publishedVersion)
- PubMed (publishedVersion)
- PORTO@Iris (submittedVersion)
- PORTO Publications Open Repository TOrino (Politecnico di Torino) (submittedVersion)
- Topics
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Keywords
- MoS2, reduced graphene oxide, supercapacitor electrodes, hybrid aerogels, specific capacitance, cycling stability, MoS2/rGO composite
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