Cited by 142Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsFuel Cells and Related Materials

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Amorphous Phosphorus-Incorporated Cobalt Molybdenum Sulfide on Carbon Cloth: An Efficient and Stable Electrocatalyst for Enhanced Overall Water Splitting over Entire pH Values

Ray, Chaiti, Lee, Su Chan, Sankar, Kalimuthu Vijaya, Jin, Bingjun, Lee, Jungpyo, Park, Jong Hyeok, Jun, Seong Chan·2017·ACS Applied Materials & Interfaces

DOI 10.1021/acsami.7b11192

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Abstract

The development of economical, proficient, and highly stable catalysts to substitute the expensive noble metal electrodes for electrocatalytic water-splitting applications is exceedingly desirable. In this context, the most fascinating and challenging approach is the rational design of a nanocomposite encompassing multiple components with unique functionalities. Herein, we describe the fabrication of a strongly catalytic and superb durable phosphorus-incorporated cobalt molybdenum sulfide electrocatalyst grown on carbon cloth (P-CoMoS/CC). The hybrid material exhibited excellent activity for hydrogen and oxygen evolution reactions over a wide range of pH (1-14) with extremely high stability (∼90% retention of the initial current density) after 24 h of electrolysis. Importantly, when P-CoMoS/CC was used as both cathode and anode for overall water splitting, a very low cell voltage of 1.54 V is required to attain the 10 mA cm -2 current density, and the hybrid material exhibited a long-term stability (89.8% activity retention after 100 h). The outstanding overall water-splitting performance compared to an electrolyzer consisting of the noble-metal-based catalysts Pt/C and RuO 2 makes P-CoMoS one of the most efficient earth-abundant water-splitting catalysts. Phosphorus incorporation was proved to be a vital aspect for the improved charge-transfer properties and catalytic durability of the P-CoMoS/CC catalyst.

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Self-citation
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Authors: Ray, C., Lee, S. C., Sankar, K. V., Jin, B., Lee, J., Park, J. H., & Jun, S. C.
Affiliations: Yonsei University (KR)
Corresponding author: Jun, Seong Chan
ORCID: Ray, Chaiti
Sankar, Kalimuthu Vijaya
Jin, Bingjun
Lee, Jungpyo
Park, Jong Hyeok
Jun, Seong Chan
Venue: ACS Applied Materials & Interfaces
Publisher: American Chemical Society (ACS)
Published: 2017-10-23
Volume: 9
Issue: 43
Pages: 37739-37749
ISSN: 1944-8244 (ISSN-L)
1944-8252
DOI: 10.1021/acsami.7b11192
OpenAlex: W2763770968
Cited by: 142
References: 70
Citations by year: 2026: 4 · 2025: 10 · 2024: 12 · 2023: 18 · 2022: 19 · 2021: 20 · 2020: 28 · 2019: 16 · 2018: 15
FWCI: 4.33
Type: journal article
Language: en
Open access: closed
Locations: ACS Applied Materials & Interfaces (publishedVersion)
PubMed (publishedVersion)
Funders: Ministry of Education, Science and Technology (2009-0093823)
Ministry of Environment (2016002130005)
Ministry of Science, ICT and Future Planning (2015R1A5A1037668)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Keywords: cobalt molybdenum sulfide, phosphorus incorporation, carbon cloth, overall water splitting, hydrogen evolution reaction, oxygen evolution reaction, electrocatalysts, earth-abundant catalysts, charge transfer, catalyst stability, nanocomposites

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Amorphous Phosphorus-Incorporated Cobalt Molybdenum Sulfide on Carbon Cloth: An Efficient and Stable Electrocatalyst for Enhanced Overall Water Splitting over Entire pH Values

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