The DOI matches its Crossref record; 33 of the 33 references it cites were found in a registry or an index.
3D Fiber-Network-Reinforced Bicontinuous Composite Solid Electrolyte for Dendrite-free Lithium Metal Batteries
Abstract
Replacement of flammable organic liquid electrolytes with solid Li + conductors is a promising approach to realize excellent performance of Li metal batteries. However, ceramic electrolytes are either easily reduced by Li metal or penetrated by Li dendrites through their grain boundaries, and polymer electrolytes are also faced with instability on the electrode/electrolyte interface and weak mechanical property. Here, we report a three-dimensional fiber-network-reinforced bicontinuous solid composite electrolyte with flexible Li + -conductive network (lithium aluminum titanium phosphate (LATP)/polyacrylonitrile), which helps to enhance electrochemical stability on the electrode/electrolyte interface by isolating Li and LATP and suppress Li dendrites growth by mechanical reinforcement of fiber network for the composite solid electrolyte. The composite electrolyte shows an excellent electrochemical stability after 15 days of contact with Li metal and has an enlarged tensile strength (10.72 MPa) compared to the pure poly(ethylene oxide)–bistrifluoromethanesulfonimide lithium salt electrolyte, leading to a long-term stability and safety of the Li symmetric battery with a current density of 0.3 mA cm –2 for 400 h. In addition, the composite electrolyte also shows good electrochemical and thermal stability. These results provide such fiber-reinforced membranes that present stable electrode/electrolyte interface and suppress lithium dendrite growth for high-safety all-solid-state Li metal batteries.
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Citations
Cites
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Negating interfacial impedance in garnet-based solid-state Li metal batteries
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Fluoroethylene Carbonate Additives to Render Uniform Li Deposits in Lithium Metal Batteries
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Self-citation
Cited by
Liang, J.-Y., Zeng, X.-X., Zhang, X.-D., Zuo, T.-T., Yan, M., Yin, Y.-X., Shi, J.-L., Wu, X.-W., Guo, Y.-G., & Wan, L.-J. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03517 · Cited by 404
Recent progress on solid-state hybrid electrolytes for solid-state lithium batteries
Liang, J., Luo, J., Sun, Q., Yang, X., Li, R., & Sun, X. (2019) · Energy Storage Materials · doi:10.1016/j.ensm.2019.06.021 · Cited by 365
Mobile Ions in Composite Solids
Zou, Z., Li, Y., Lu, Z., Wang, D., Cui, Y., Guo, B., Li, Y., Liang, X., Feng, J., Li, H., et al. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00760 · Cited by 348
Self-citationElectrolytes in Organic Batteries
Li, M., Hicks, R. P., Chen, Z., Luo, C., Guo, J., Wang, C., & Xu, Y. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00374 · Cited by 303
Metadata
- Authors
- Li, D., Chen, L., Wang, T., & Fan, L.-Z.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-02-20
- Volume
- 10
- Issue
- 8
- Pages
- 7069-7078
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2785887360
- Cited by
- 398
- References
- 33
- FWCI
- 16.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, D., Chen, L., Wang, T., & Fan, L.-Z. (2018). 3D Fiber-Network-Reinforced Bicontinuous Composite Solid Electrolyte for Dendrite-free Lithium Metal Batteries. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b18123
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