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g-C3N4/NiAl-LDH 2D/2D Hybrid Heterojunction for High-Performance Photocatalytic Reduction of CO2 into Renewable Fuels
Open accessAbstract
2D/2D interface heterostructures of g-C 3 N 4 and NiAl-LDH are synthesized utilizing strong electrostatic interactions between positively charged 2D NiAl-LDH sheets and negatively charged 2D g-C 3 N 4 nanosheets. This new 2D/2D interface heterojunction showed remarkable performance for photocatalytic CO 2 reduction to produce renewable fuels such as CO and H 2 under visible-light irradiation, far superior to that of either single phase g-C 3 N 4 or NiAl-LDH nanosheets. The enhancement of photocatalytic activity could be attributed mainly to the excellent interfacial contact at the heterojunction of g-C 3 N 4 /NiAl-LDH, which subsequently results in suppressed recombination, and improved transfer and separation of photogenerated charge carriers. In addition, the optimal g-C 3 N 4 /NiAl-LDH nanocomposite possessed high photostability after successive experimental runs with no obvious change in the production of CO from CO 2 reduction. Our findings regarding the design, fabrication and photophysical properties of 2D/2D heterostructure systems may find use in other photocatalytic applications including H 2 production and water purification.
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Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Gao, Z., Wang, J., Li, Z., Yang, W., Wang, B., Hou, M., He, Y., Liu, Q., Mann, T., Yang, P., et al. (2011) · Chemistry of Materials · doi:10.1021/cm200975x · Cited by 542
Cited by
Cocatalysts for Selective Photoreduction of CO2into Solar Fuels
Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Z‐Scheme Photocatalytic Systems for Carbon Dioxide Reduction: Where Are We Now?
Zhang, W., Mohamed, A. R., & Ong, W. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201914925 · Cited by 667
Akhundi, A., Habibi-Yangjeh, A., Abitorabi, M., & Rahim Pouran, S. (2019) · Catalysis Reviews · doi:10.1080/01614940.2019.1654224 · Cited by 526
Vu, N., Kaliaguine, S., & Do, T. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901825 · Cited by 445
Heterostructured Catalysts for Electrocatalytic and Photocatalytic Carbon Dioxide Reduction
Prabhu, P., Jose, V., & Lee, J. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201910768 · Cited by 432
Metadata
- Authors
- Tonda, S., Kumar, S., Bhardwaj, M., Yadav, P., & Ogale, S.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-01-11
- Volume
- 10
- Issue
- 3
- Pages
- 2667-2678
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2779251897
- Cited by
- 556
- References
- 4
- FWCI
- 11.53
- Type
- journal article
- Language
- en
- Open access
- green
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- Tonda, S., Kumar, S., Bhardwaj, M., Yadav, P., & Ogale, S. (2018). g-C3N4/NiAl-LDH 2D/2D Hybrid Heterojunction for High-Performance Photocatalytic Reduction of CO2 into Renewable Fuels. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b18835
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