The DOI matches its Crossref record; 35 of the 35 references it cites were found in a registry or an index.
Stabilizing the Interface of NASICON Solid Electrolyte against Li Metal with Atomic Layer Deposition
Abstract
Solid-state batteries have been considered as one of the most promising next-generation energy storage systems because of their high safety and energy density. Solid-state electrolytes are the key component of the solid-state battery, which exhibit high ionic conductivity, good chemical stability, and wide electrochemical windows. LATP [Li 1.3 Al 0.3 Ti 1.7 (PO 4 ) 3 ] solid electrolyte has been widely investigated for its high ionic conductivity. Nevertheless, the chemical instability of LATP against Li metal has hindered its application in solid-state batteries. Here, we propose that atomic layer deposition (ALD) coating on LATP surfaces is able to stabilize the LATP/Li interface by reducing the side reactions. In comparison with bare LATP, the Al 2 O 3 -coated LATP by ALD exhibits a stable cycling behavior with smaller voltage hysteresis for 600 h, as well as small resistance. More importantly, on the basis of advanced characterizations such as high-resolution transmission electron spectroscope-electron energy loss spectroscopy, the lithium penetration into the LATP bulk and Ti 4+ reduction are significantly limited. The results suggest that ALD is very effective in improving solid-state electrolyte/electrode interface stability.
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Cites
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Self-citationElectrolytes for solid-state lithium rechargeable batteries: recent advances and perspectives
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Cited by
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Physicochemical Concepts of the Lithium Metal Anode in Solid-State Batteries
Krauskopf, T., Richter, F. H., Zeier, W. G., & Janek, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00431 · Cited by 892
Lithium metal anodes: Present and future
Wang, R., Cui, W., Chu, F., & Wu, F. (2020) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2019.12.024 · Cited by 544
Liang, J.-Y., Zeng, X.-X., Zhang, X.-D., Zuo, T.-T., Yan, M., Yin, Y.-X., Shi, J.-L., Wu, X.-W., Guo, Y.-G., & Wan, L.-J. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03517 · Cited by 404
Recent progress on solid-state hybrid electrolytes for solid-state lithium batteries
Liang, J., Luo, J., Sun, Q., Yang, X., Li, R., & Sun, X. (2019) · Energy Storage Materials · doi:10.1016/j.ensm.2019.06.021 · Cited by 365
Self-citation
Metadata
- Authors
- Liu, Y., Sun, Q., Zhao, Y., Wang, B., Kaghazchi, P., Adair, K. R., Li, R., Zhang, C., Liu, J., Kuo, L.-Y., Hu, Y., Sham, T.-K., Zhang, L., Yang, R., Lu, S., Song, X., & Sun, X.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-08-24
- Volume
- 10
- Issue
- 37
- Pages
- 31240-31248
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2888761391
- Cited by
- 312
- References
- 35
- FWCI
- 9.69
- Type
- journal article
- Language
- en
- Open access
- closed
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