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A Review on Challenges and Successes in Atomic-Scale Design of Catalysts for Electrochemical Synthesis of Hydrogen Peroxide
Open accessAbstract
Hydrogen peroxide is a valuable chemical oxidant with a wide range of applications in a variety of industrial processes, especially in water sanitization. Electrochemical synthesis of hydrogen peroxide (H 2 O 2 ) through a two-electron oxygen reduction reaction (2e-ORR) or a two-electron water oxidation reaction (2e-WOR) has emerged as an appealing process for onsite production of this chemically valuable oxidant. On-site produced H 2 O 2 can be applied for wastewater treatment in remote locations or any applications where H 2 O 2 is needed as an oxidizing agent. This Review studies the theoretical efforts in understanding the challenges in catalysis for electrochemical synthesis of H 2 O 2 as well as providing design principles for more efficient catalyst materials.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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Self-citationUniversality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
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Self-citationComputational high-throughput screening of electrocatalytic materials for hydrogen evolution
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How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels
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Self-citationHydrogen Peroxide Synthesis: An Outlook beyond the Anthraquinone Process
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Alloys of platinum and early transition metals as oxygen reduction electrocatalysts
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Understanding Catalytic Activity Trends in the Oxygen Reduction Reaction
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Self-citation
Cited by
Hydroxyl radicals in anodic oxidation systems: generation, identification and quantification
Xie, J., Zhang, C., & Waite, T. D. (2022) · Water Research · doi:10.1016/j.watres.2022.118425 · Cited by 303
Metadata
- Authors
- Siahrostami, S., Villegas, S. J., Bagherzadeh Mostaghimi, A. H., Back, S., Farimani, A. B., Wang, H., Persson, K. A., & Montoya, J.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-06-10
- Volume
- 10
- Issue
- 14
- Pages
- 7495-7511
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W3034591340
- Cited by
- 503
- References
- 117
- FWCI
- 11.42
- Type
- journal article
- Language
- en
- Open access
- green
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- Siahrostami, S., Villegas, S. J., Bagherzadeh Mostaghimi, A. H., Back, S., Farimani, A. B., Wang, H., Persson, K. A., & Montoya, J. (2020). A Review on Challenges and Successes in Atomic-Scale Design of Catalysts for Electrochemical Synthesis of Hydrogen Peroxide. ACS Catalysis. https://doi.org/10.1021/acscatal.0c01641
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