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Elucidating the Roles of Electric Fields in Catalysis: A Perspective
Abstract
This Perspective illustrates how the presence of internal and external electric fields can affect catalytic activity and selectivity, with a focus on heterogeneous catalysts. Specifically, experimental investigations of the electric field influence on catalyst selectivity in pulsed field mass desorption microscopes, scanning tunneling microscopes, probe–bed–probe reactors, continuous-circuit reactors, and capacitor reactors are described. Through these examples, we show how the electric field, whether externally applied or intrinsically present, can affect the behavior of a wide number of materials relevant to catalysis. We review some of the theoretical methods that have been used to elucidate the influence of external electric fields on catalytic reactions, as well as the application of such methods to selective methane activation. In doing so, we illustrate the breadth of possibilities in field-assisted catalysis.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
Nørskov, J. K., Rossmeisl, J., Logadottir, A., Lindqvist, L., Kitchin, J. R., Bligaard, T., & Jónsson, H. (2004) · The Journal of Physical Chemistry B · doi:10.1021/jp047349j · Cited by 13,153
Current Status of Transition-State Theory
Truhlar, D. G., Garrett, B. C., & Klippenstein, S. J. (1996) · The Journal of Physical Chemistry · doi:10.1021/jp953748q · Cited by 2,279
Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
Ulissi, Z. W., Medford, A. J., Bligaard, T., & Nørskov, J. K. (2017) · Nature Communications · doi:10.1038/ncomms14621 · Cited by 614
The radical mechanism of biological methane synthesis by methyl-coenzyme M reductase
Wongnate, T., Sliwa, D., Ginovska, B., Smith, D., Wolf, M. W., Lehnert, N., Raugei, S., & Ragsdale, S. W. (2016) · Science · doi:10.1126/science.aaf0616 · Cited by 170
Assessing a First-Principles Model of an Electrochemical Interface by Comparison with Experiment
Steinmann, S. N., & Sautet, P. (2016) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.6b01938 · Cited by 120
Cited by
Microwave-initiated catalytic deconstruction of plastic waste into hydrogen and high-value carbons
Jie, X., Li, W., Slocombe, D., Gao, Y., Banerjee, I., Gonzalez-Cortes, S., Yao, B., AlMegren, H., Alshihri, S., Dilworth, J., et al. (2020) · Nature Catalysis · doi:10.1038/s41929-020-00518-5 · Cited by 611
Waegele, M. M., Gunathunge, C. M., Li, J., & Li, X. (2019) · The Journal of Chemical Physics · doi:10.1063/1.5124878 · Cited by 423
Shaik, S., Danovich, D., Joy, J., Wang, Z., & Stuyver, T. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c05128 · Cited by 373
Metadata
- Authors
- Che, F., Gray, J. T., Ha, S., Kruse, N., Scott, S. L., & McEwen, J.-S.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-04-02
- Volume
- 8
- Issue
- 6
- Pages
- 5153-5174
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2795948396
- Cited by
- 381
- References
- 6
- FWCI
- 10.57
- Type
- journal article
- Language
- en
- Open access
- closed
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- Che, F., Gray, J. T., Ha, S., Kruse, N., Scott, S. L., & McEwen, J.-S. (2018). Elucidating the Roles of Electric Fields in Catalysis: A Perspective. ACS Catalysis. https://doi.org/10.1021/acscatal.7b02899
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