Cited by 611Thermochemical Biomass Conversion ProcessesCatalysts for Methane ReformingMicrowave-Assisted Synthesis and Applications

Microwave-initiated catalytic deconstruction of plastic waste into hydrogen and high-value carbons

Jie, Xiangyu, Li, Weisong, Slocombe, Daniel, Gao, Yige, Banerjee, Ira, Gonzalez-Cortes, Sergio, Yao, Benzhen, AlMegren, Hamid +5 more·2020·Nature Catalysis

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Crossref · 10.1038/s41929-020-00518-5

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3 of 3 references verified0 citation errors · 0 not checkable

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  • The technique achieved a hydrogen yield of 55.6 mmol/g plastic (reaching 97% of theoretical hydrogen mass), with a hydrogen concentration of about 90 vol% in the effluent gas.

    “The technique achieved a hydrogen yield of 55.6 mmol/g plastic (reaching 97% of the theoretical hydrogen mass), with a hydrogen concentration of about 90 vol% in the effluent gas.”
  • Fe-based catalyst (FeAlOx) efficiently converts shredded plastic waste into hydrogen and multiwalled carbon nanotubes (MWCNTs) within 30-90 s.

    “Jie and colleagues utilized an Fe-based catalyst (FeAlO x ) to efficiently convert shredded plastic waste into hydrogen and multiwalled carbon nanotubes (MWCNTs) within 30-90 s [74] .”
  • Continuous feeding achieved a carbon production rate of 1,560 mg C/g plastic/g Catalyst, with MWCNT purity exceeding 92 wt%.

    “Continuous feeding achieved a carbon production rate of 1,560 mg C/g plastic /g Catalyst , with MWCNT purity exceeding 92 wt%.”
  • Using inexpensive iron-based catalysts as microwave sensors, a rapid catalytic decomposition process of plastic was initiated for 30-90 s, converting mechanically crushed commercial plastics into 55.6 mmol/g high yield hydrogen and multi walled carbon nanotubes.

    “Using inexpensive iron-based catalysts as microwave sensors, a rapid catalytic decomposition process of plastic was initiated for 30-90 s, converting mechanically crushed commercial plastics into 55.6 mmol/g high yield hydrogen and multi walled carbon nanotubes (Jie et al. 2020).”

    From Conversion of waste plastics into value-added carbon materials (2023) · cites this paper as Jie et al. 2020

  • Microwave carbonization is a new method for efficiently and rapidly converting waste plastics into carbon nanotubes and hydrogen.

    “Recently, microwave carbonization has attracted much attention as a new method for efficiently and rapidly converting waste plastics into carbon nanotubes and hydrogen (Jie et al. 2020).”

    From Conversion of waste plastics into value-added carbon materials (2023) · cites this paper as Jie et al. 2020

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Authors
Jie, X., Li, W., Slocombe, D., Gao, Y., Banerjee, I., Gonzalez-Cortes, S., Yao, B., AlMegren, H., Alshihri, S., Dilworth, J., Thomas, J., Xiao, T., & Edwards, P.
Affiliations
  • University of Oxford (GB)
  • Tianjin University (CN)
  • Cardiff University (GB)
  • King Abdulaziz City for Science and Technology (SA)
  • University of Cambridge (GB)
Corresponding author
  • Thomas, John
  • Xiao, Tiancun
  • Edwards, Peter
Venue
Nature Catalysis
Published
2020-10-12
Volume
3
Issue
11
Pages
902-912
ISSN
2520-1158 (ISSN-L)
OpenAlex
W3094916216
Cited by
611
References
3
Citations by year
2026: 94 · 2025: 141 · 2024: 110 · 2023: 114 · 2022: 100 · 2021: 51 · 2020: 1
FWCI
20.90
Type
journal article
Language
en
Open access
closed
Locations
  • Nature Catalysis (publishedVersion)
  • ORCA Online Research @Cardiff (Cardiff University) (acceptedVersion)
  • ORCA Online Research @Cardiff (Cardiff University) (submittedVersion)
Funders
King Abdulaziz City for Science and Technology (KOPRC I/II)
Topics
  • Physical Sciences › Engineering › Biomedical Engineering › Thermochemical Biomass Conversion Processes
  • Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
  • Physical Sciences › Chemistry › Organic Chemistry › Microwave-Assisted Synthesis and Applications
Keywords
plastic waste, microwave-assisted catalysis, hydrogen production, multi-walled carbon nanotubes, iron catalysts, microwave susceptors, plastisphere

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