The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Earth-Abundant Oxygen Electrocatalysts for Alkaline Anion-Exchange-Membrane Water Electrolysis: Effects of Catalyst Conductivity and Comparison with Performance in Three-Electrode Cells
Open accessAbstract
Anion exchange membrane (AEM) electrolysis is a promising technology to produce hydrogen through the splitting of pure water. In contrast to proton-exchange-membrane (PEM) technology, which requires precious-metal oxide anodes, AEM systems allow for the use of earth-abundant anode catalysts. Here we report a study of first-row transition-metal (oxy)hydroxide/oxide catalyst powders for application in AEM devices and compare physical properties and performance to benchmark IrO x catalysts as well as typical catalysts for alkaline electrolyzers. We show that the catalysts’ oxygen-evolution activity measured in alkaline electrolyte using a typical three-electrode cell is a poor indicator of performance in the AEM system. The best oxygen-evolution-reaction (OER) catalysts in alkaline electrolyte, NiFeO x H y oxyhydroxides, are the worst in AEM electrolysis devices where a solid alkaline electrolyte is used along with a pure water feed. NiCoO x -based catalysts show the best performance in AEM electrolysis. The performance can be further improved by adding Fe species to the particle surface. We attribute the differences in performance in part to differences in the electrical conductivity of the catalyst phases, which are also measured and reported.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Anion-exchange membranes in electrochemical energy systems
Varcoe, J. R., Atanassov, P., Dekel, D. R., Herring, A. M., Hickner, M. A., Kohl, P. A., Kucernak, A. R., Mustain, W. E., Nijmeijer, K., Scott, K., et al. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01303d · Cited by 2,051
First implementation of alkaline polymer electrolyte water electrolysis working only with pure water
Xiao, L., Zhang, S., Pan, J., Yang, C., He, M., Zhuang, L., & Lu, J. (2012) · Energy & Environmental Science · doi:10.1039/c2ee22146b · Cited by 313
Cited by
Oxygen Evolution Reaction in Alkaline Environment: Material Challenges and Solutions
Xie, X., Du, L., Yan, L., Park, S., Qiu, Y., Sokolowski, J., Wang, W., & Shao, Y. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202110036 · Cited by 792
Fe-Based Electrocatalysts for Oxygen Evolution Reaction: Progress and Perspectives
Feng, C., Faheem, M. B., Fu, J., Xiao, Y., Li, C., & Li, Y. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05445 · Cited by 587
Self-citationJiang, W., Faid, A. Y., Gomes, B. F., Galkina, I., Xia, L., Lobo, C. M. S., Desmau, M., Borowski, P., Hartmann, H., Maljusch, A., et al. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202203520 · Cited by 161
NiFe2O4 hierarchical nanoparticles as electrocatalyst for anion exchange membrane water electrolysis
Martinez-Lazaro, A., Caprì, A., Gatto, I., Ledesma-García, J., Rey-Raap, N., Arenillas, A., Espinosa-Lagunes, F. I., Baglio, V., & Arriaga, L. G. (2023) · Journal of Power Sources · doi:10.1016/j.jpowsour.2022.232417 · Cited by 54
Aerogel-derived nickel-iron oxide catalysts for oxygen evolution reaction in alkaline media
Osmieri, L., Yu, H., Hermann, R. P., Kreider, M. E., Meyer, H. M., Kropf, A. J., Park, J. H., Alia, S. M., Cullen, D. A., Myers, D. J., et al. (2024) · Applied Catalysis B: Environment and Energy · doi:10.1016/j.apcatb.2024.123843 · Cited by 34
Metadata
- Authors
- Xu, D., Stevens, M. B., Cosby, M. R., Oener, S. Z., Smith, A. M., Enman, L. J., Ayers, K. E., Capuano, C. B., Renner, J. N., Danilovic, N., Li, Y., Wang, H., Zhang, Q., & Boettcher, S. W.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-11-15
- Volume
- 9
- Issue
- 1
- Pages
- 7-15
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2900744414
- Cited by
- 331
- References
- 3
- FWCI
- 4.24
- Type
- journal article
- Language
- en
- Open access
- green
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- Xu, D., Stevens, M. B., Cosby, M. R., Oener, S. Z., Smith, A. M., Enman, L. J., Ayers, K. E., Capuano, C. B., Renner, J. N., Danilovic, N., Li, Y., Wang, H., Zhang, Q., & Boettcher, S. W. (2019). Earth-Abundant Oxygen Electrocatalysts for Alkaline Anion-Exchange-Membrane Water Electrolysis: Effects of Catalyst Conductivity and Comparison with Performance in Three-Electrode Cells. ACS Catalysis. https://doi.org/10.1021/acscatal.8b04001
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