The DOI matches its Crossref record; 43 of the 43 references it cites were found in a registry or an index.
Redox Catalysis Facilitates Lignin Depolymerization
Open accessAbstract
Lignin is a recalcitrant and underexploited natural feedstock for aromatic commodity chemicals, and its degradation generally requires the use of high temperatures and harsh reaction conditions. Herein we present an ambient temperature one-pot process for the controlled oxidation and depolymerization of this potent resource. Harnessing the potential of electrocatalytic oxidation in conjugation with our photocatalytic cleavage methodology, we have developed an operationally simple procedure for selective fragmentation of β-O-4 bonds with excellent mass recovery, which provides a unique opportunity to expand the existing lignin usage from energy source to commodity chemicals and synthetic building block source.
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Cites
The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
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Lignin Biosynthesis and Structure
Vanholme, R., Demedts, B., Morreel, K., Ralph, J., & Boerjan, W. (2010) · Plant Physiology · doi:10.1104/pp.110.155119 · Cited by 2,664
Catalytic conversion of biomass to biofuels
Alonso, D. M., Bond, J. Q., & Dumesic, J. A. (2010) · Green Chemistry · doi:10.1039/c004654j · Cited by 2,333
Redox catalysis in organic electrosynthesis: basic principles and recent developments
Francke, R., & Little, R. D. (2014) · Chemical Society Reviews · doi:10.1039/c3cs60464k · Cited by 1,930
Thermochemistry of Proton-Coupled Electron Transfer Reagents and its Implications
Warren, J. J., Tronic, T. A., & Mayer, J. M. (2010) · Chemical Reviews · doi:10.1021/cr100085k · Cited by 1,692
Lignins: Natural polymers from oxidative coupling of 4-hydroxyphenyl- propanoids
Ralph, J., Lundquist, K., Brunow, G., Lu, F., Kim, H., Schatz, P. F., Marita, J. M., Hatfield, R. D., Ralph, S. A., Christensen, J. H., et al. (2004) · Phytochemistry Reviews · doi:10.1023/b:phyt.0000047809.65444.a4 · Cited by 1,660
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Lignin Depolymerization and Conversion: A Review of Thermochemical Methods
Pandey, M. P., & Kim, C. S. (2011) · Chemical Engineering & Technology · doi:10.1002/ceat.201000270 · Cited by 1,419
Formaldehyde stabilization facilitates lignin monomer production during biomass depolymerization
Shuai, L., Amiri, M. T., Questell-Santiago, Y. M., Héroguel, F., Li, Y., Kim, H., Meilan, R., Chapple, C., Ralph, J., & Luterbacher, J. S. (2016) · Science · doi:10.1126/science.aaf7810 · Cited by 1,404
Formic-acid-induced depolymerization of oxidized lignin to aromatics
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Cited by
Wu, X., Fan, X., Xie, S., Lin, J., Cheng, J., Zhang, Q., Chen, L., & Wang, Y. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0148-8 · Cited by 649
Tay, N. E. S., Lehnherr, D., & Rovis, T. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00384 · Cited by 518
Singh, A. K., Bilal, M., Iqbal, H. M. N., Meyer, A. S., & Raj, A. (2021) · Science of The Total Environment · doi:10.1016/j.scitotenv.2021.145988 · Cited by 205
Metadata
- Authors
- Bosque, I., Magallanes, G., Rigoulet, M., Kärkäs, M. D., & Stephenson, C. R. J.
- Venue
- ACS Central Science
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-06-07
- Volume
- 3
- Issue
- 6
- Pages
- 621-628
- ISSN
- 2374-7943 (ISSN-L)
- 2374-7951
- OpenAlex
- W2624022514
- Cited by
- 293
- References
- 43
- FWCI
- 10.94
- Type
- journal article
- Language
- en
- Open access
- diamond
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- Bosque, I., Magallanes, G., Rigoulet, M., Kärkäs, M. D., & Stephenson, C. R. J. (2017). Redox Catalysis Facilitates Lignin Depolymerization. ACS Central Science. https://doi.org/10.1021/acscentsci.7b00140
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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