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Unveiling the Origin of Alloy-Seeded and Nondendritic Growth of Zn for Rechargeable Aqueous Zn Batteries
Abstract
Rechargeable aqueous zinc anodes have gained tremendous attention because of their merits of intrinsic safety, low cost, and high theoretical volumetric capacity (5854 mAh cm –3 for Zn metal). In aqueous electrolytes, zinc anodes suffer from severe dendritic metal deposition. The regulation of Zn by inducing Zn-alloying metals has been reported. However, the underlying mechanisms have remained elusive. Here, for the first time, we did a comprehensive analysis to elucidate the mechanisms for the seeded and nondendritic growth of Zn on alloy anodes. We achieved uniform Zn deposition by introducing a Zn-alloying and soluble metal, Ag, on Zn anodes. Due to a shift of thermodynamic potential and the spatial confinement, the Ag-modified Zn anode exhibited improved overall cycling performance compared with previous deep-cycle Zn anodes. Furthermore, the seeded Zn deposition was visualized in operando for the first time using an optical microscope. The alloy-seeding design principle here can potentially be applied to improve the rechargeability of other metal anodes.
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Citations
Cites
Atomic structure of sensitive battery materials and interfaces revealed by cryo–electron microscopy
Li, Y., Li, Y., Pei, A., Yan, K., Sun, Y., Wu, C.-L., Joubert, L.-M., Chin, R., Koh, A. L., Yu, Y., et al. (2017) · Science · doi:10.1126/science.aam6014 · Cited by 1,547
Cited by
Yuan, L., Hao, J., Kao, C.-C., Wu, C., Liu, H.-K., Dou, S.-X., & Qiao, S.-Z. (2021) · Energy & Environmental Science · doi:10.1039/d1ee02021h · Cited by 628
Zinc Anode for Mild Aqueous Zinc-Ion Batteries: Challenges, Strategies, and Perspectives
Yang, J., Yin, B., Sun, Y., Pan, H., Sun, W., Jia, B., Zhang, S., & Ma, T. (2022) · Nano-Micro Letters · doi:10.1007/s40820-021-00782-5 · Cited by 584
Recent Progress on Zn Anodes for Advanced Aqueous Zinc‐Ion Batteries
Nie, C., Wang, G., Wang, D., Wang, M., Gao, X., Bai, Z., Wang, N., Yang, J., Xing, Z., & Dou, S. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300606 · Cited by 561
Zn-based batteries for sustainable energy storage: strategies and mechanisms
Tang, L., Peng, H., Kang, J., Chen, H., Zhang, M., Liu, Y., Kim, D. H., Liu, Y., & Lin, Z. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00295k · Cited by 548
Xue, P., Guo, C., Li, L., Li, H., Luo, D., Tan, L., & Chen, Z. (2022) · Advanced Materials · doi:10.1002/adma.202110047 · Cited by 259
Metadata
- Authors
- Zhang, Y., Howe, J. D., Ben-Yoseph, S., Wu, Y., & Liu, N.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-01-06
- Volume
- 6
- Issue
- 2
- Pages
- 404-412
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W3118963734
- Cited by
- 262
- References
- 1
- FWCI
- 14.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, Y., Howe, J. D., Ben-Yoseph, S., Wu, Y., & Liu, N. (2021). Unveiling the Origin of Alloy-Seeded and Nondendritic Growth of Zn for Rechargeable Aqueous Zn Batteries. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.0c02343
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