The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Strain Effect in Bimetallic Electrocatalysts in the Hydrogen Evolution Reaction
Abstract
Unravelling the electrocatalytic activity origins of bimetallic nanomaterials is of great importance, yet fundamentally challenging. One of the main reasons for this is that the interactive contributions from geometric and electronic effects to enhancements in reaction activity are difficult to distinguish from one another. Here, on well-defined Ru–Pt core–shell (Ru@Pt) and homogeneous alloy (RuPt) model electrocatalysts, we are able to isolate these two effects. Furthermore, we observe the dominant role of strain in the intrinsic activity of the alkaline hydrogen evolution reaction. In the Ru@Pt icosahedral nanostructure, the highly strained Pt shells effectively accommodate the interfacial lattice mismatch from a face-centered cubic structured Ru core. This unique property leads to a weak binding of hydrogen and optimal interaction with hydroxyl species during the reaction, thus leading to an enhanced apparent activity of Ru@Pt.
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Cites
Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
Subbaraman, R., Tripkovic, D., Strmcnik, D., Chang, K.-C., Uchimura, M., Paulikas, A. P., Stamenkovic, V., & Markovic, N. M. (2011) · Science · doi:10.1126/science.1211934 · Cited by 3,135
Platinum single-atom and cluster catalysis of the hydrogen evolution reaction
Cheng, N., Stambula, S., Wang, D., Banis, M. N., Liu, J., Riese, A., Xiao, B., Li, R., Sham, T.-K., Liu, L.-M., et al. (2016) · Nature Communications · doi:10.1038/ncomms13638 · Cited by 2,072
Hydrogen Oxidation and Evolution Reaction Kinetics on Platinum: Acid vs Alkaline Electrolytes
Sheng, W., Gasteiger, H. A., & Shao-Horn, Y. (2010) · Journal of The Electrochemical Society · doi:10.1149/1.3483106 · Cited by 1,829
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
Improving the hydrogen oxidation reaction rate by promotion of hydroxyl adsorption
Strmcnik, D., Uchimura, M., Wang, C., Subbaraman, R., Danilovic, N., van der Vliet, D., Paulikas, A. P., Stamenkovic, V. R., & Markovic, N. M. (2013) · Nature Chemistry · doi:10.1038/nchem.1574 · Cited by 1,426
Sheng, W., Myint, M., Chen, J. G., & Yan, Y. (2013) · Energy & Environmental Science · doi:10.1039/c3ee00045a · Cited by 1,202
Nanostructured Pt-alloy electrocatalysts for PEM fuel cell oxygen reduction reaction
Bing, Y., Liu, H., Zhang, L., Ghosh, D., & Zhang, J. (2010) · Chemical Society Reviews · doi:10.1039/b912552c · Cited by 1,154
Sheng, W., Zhuang, Z., Gao, M., Zheng, J., Chen, J. G., & Yan, Y. (2015) · Nature Communications · doi:10.1038/ncomms6848 · Cited by 1,136
Strain-controlled electrocatalysis on multimetallic nanomaterials
Luo, M., & Guo, S. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.59 · Cited by 1,115
High Electrocatalytic Hydrogen Evolution Activity of an Anomalous Ruthenium Catalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Jaroniec, M., & Qiao, S.-Z. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b11291 · Cited by 1,110
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Cited by
Recent Advances and Prospective in Ruthenium-Based Materials for Electrochemical Water Splitting
Yu, J., He, Q., Yang, G., Zhou, W., Shao, Z., & Ni, M. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b02457 · Cited by 789
Strategies for design of electrocatalysts for hydrogen evolution under alkaline conditions
Wang, X., Zheng, Y., Sheng, W., Xu, Z. J., Jaroniec, M., & Qiao, S.-Z. (2020) · Materials Today · doi:10.1016/j.mattod.2019.12.003 · Cited by 533
Self-citationHeteroatom-doped transition metal electrocatalysts for hydrogen evolution reaction
Jin, H., Liu, X., Chen, S., Vasileff, A., Li, L., Jiao, Y., Song, L., Zheng, Y., & Qiao, S.-Z. (2019) · ACS Energy Letters · doi:10.1021/acsenergylett.9b00348 · Cited by 469
Self-citationZhu, S., Qin, X., Xiao, F., Yang, S., Xu, Y., Tan, Z., Li, J., Yan, J., Chen, Q., Chen, M., et al. (2021) · Nature Catalysis · doi:10.1038/s41929-021-00663-5 · Cited by 436
Tan, H., Tang, B., Lu, Y., Ji, Q., Lv, L., Duan, H., Li, N., Wang, Y., Feng, S., Li, Z., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-29710-w · Cited by 390
Metadata
- Authors
- Wang, X., Zhu, Y., Vasileff, A., Jiao, Y., Chen, S., Song, L., Zheng, B., Zheng, Y., & Qiao, S.-Z.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-04-27
- Volume
- 3
- Issue
- 5
- Pages
- 1198-1204
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2799581409
- Cited by
- 236
- References
- 10
- FWCI
- 6.05
- Type
- journal article
- Language
- en
- Open access
- closed
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