The DOI matches its Crossref record; 28 of the 28 references it cites were found in a registry or an index.
High Rate, Selective, and Stable Electroreduction of CO2 to CO in Basic and Neutral Media
Open accessAbstract
The electroreduction of carbon dioxide (CO 2 ) to chemicals such as carbon monoxide (CO) shows great potential for renewable fuel and chemical production. Significant progress in individual performance metrics such as reaction rate, selectivity, and stability has been achieved, yet the simultaneous achievement of each of these key metrics within a single system, and in a wide range of operating conditions, has yet to be demonstrated. Here we report a composite multilayered porous electrode consisting of a polytetrafluoroethylene gas distribution layer, a conformal Ag catalyst, and a carbon current distributor. Separating the gas and current distribution functions provides endurance, and further reconstructing the catalyst to carbonate-derived Ag provides flexibility in terms of electrolyte. The resulting electrodes reduce CO 2 to CO with a Faradaic efficiency over 90% at current densities above 150 mA/cm 2, in both neutral and alkaline media for over 100 h of operation. This represents an important step toward the deployment of CO 2 electroduction systems using electrolyzer technologies.
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Cites
Covalent organic frameworks comprising cobalt porphyrins for catalytic CO 2 reduction in water
Lin, S., Diercks, C. S., Zhang, Y.-B., Kornienko, N., Nichols, E. M., Zhao, Y., Paris, A. R., Kim, D., Yang, P., Yaghi, O. M., et al. (2015) · Science · doi:10.1126/science.aac8343 · Cited by 2,644
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Self-citationEnhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
Self-citationAqueous CO2 Reduction at Very Low Overpotential on Oxide-Derived Au Nanoparticles
Chen, Y., Li, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja309317u · Cited by 1,664
What Should We Make with CO2 and How Can We Make It?
Bushuyev, O. S., De Luna, P., Dinh, C. T., Tao, L., Saur, G., van de Lagemaat, J., Kelley, S. O., & Sargent, E. H. (2018) · Joule · doi:10.1016/j.joule.2017.09.003 · Cited by 1,593
Self-citationA selective and efficient electrocatalyst for carbon dioxide reduction
Lu, Q., Rosen, J., Zhou, Y., Hutchings, G. S., Kimmel, Y. C., Chen, J. G., & Jiao, F. (2014) · Nature Communications · doi:10.1038/ncomms4242 · Cited by 1,478
Size-Dependent Electrocatalytic Reduction of CO2 over Pd Nanoparticles
Gao, D., Zhou, H., Wang, J., Miao, S., Yang, F., Wang, G., Wang, J., & Bao, X. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b00046 · Cited by 1,099
Electrolytic CO2 Reduction in a Flow Cell
Weekes, D. M., Salvatore, D. A., Reyes, A., Huang, A., & Berlinguette, C. P. (2018) · Accounts of Chemical Research · doi:10.1021/acs.accounts.8b00010 · Cited by 1,067
Nanostructured transition metal dichalcogenide electrocatalysts for CO 2 reduction in ionic liquid
Asadi, M., Kim, K., Liu, C., Addepalli, A. V., Abbasi, P., Yasaei, P., Phillips, P., Behranginia, A., Cerrato, J. M., Haasch, R., et al. (2016) · Science · doi:10.1126/science.aaf4767 · Cited by 907
Robust carbon dioxide reduction on molybdenum disulphide edges
Asadi, M., Kumar, B., Behranginia, A., Rosen, B. A., Baskin, A., Repnin, N., Pisasale, D., Phillips, P., Zhu, W., Haasch, R., et al. (2014) · Nature Communications · doi:10.1038/ncomms5470 · Cited by 766
Cited by
CO 2 electrolysis to multicarbon products at activities greater than 1 A cm −2
García de Arquer, F. P., Dinh, C.-T., Ozden, A., Wicks, J., McCallum, C., Kirmani, A. R., Nam, D.-H., Gabardo, C., Seifitokaldani, A., Wang, X., et al. (2020) · Science · doi:10.1126/science.aay4217 · Cited by 1,517
Self-citationElectrocatalytic carbon dioxide reduction: from fundamental principles to catalyst design
Zhang, X., Guo, S.-X., Gandionco, K. A., Bond, A. M., & Zhang, J. (2020) · Materials Today Advances · doi:10.1016/j.mtadv.2020.100074 · Cited by 322
Ternary Sn‐Ti‐O Electrocatalyst Boosts the Stability and Energy Efficiency of CO2 Reduction
Wen, G., Ren, B., Park, M. G., Yang, J., Dou, H., Zhang, Z., Deng, Y., Bai, Z., Yang, L., Gostick, J., et al. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202004149 · Cited by 97
Metadata
- Authors
- Dinh, C.-T., García de Arquer, F. P., Sinton, D., & Sargent, E. H.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-10-17
- Volume
- 3
- Issue
- 11
- Pages
- 2835-2840
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2896846575
- Cited by
- 348
- References
- 28
- FWCI
- 6.62
- Type
- journal article
- Language
- en
- Open access
- green
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- Dinh, C.-T., García de Arquer, F. P., Sinton, D., & Sargent, E. H. (2018). High Rate, Selective, and Stable Electroreduction of CO2 to CO in Basic and Neutral Media. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b01734
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